Bose-Einstein Condensation of Long-Lifetime Polaritons in Thermal Equilibrium
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The experimental realization of Bose-Einstein condensation (BEC) with atoms and quasiparticles has triggered wide exploration of macroscopic quantum effects. Microcavity polaritons are of particular interest because quantum phenomena such as BEC and superfluidity can be observed at elevated temperatures. However, polariton lifetimes are typically too short to permit thermal equilibration. This has led to debate about whether polariton condensation is intrinsically a nonequilibrium effect. Here we report the first unambiguous observation of BEC of optically trapped polaritons in thermal equilibrium in a high-Q microcavity, evidenced by equilibrium Bose-Einstein distributions over broad ranges of polariton densities and bath temperatures. With thermal equilibrium established, we verify that polariton condensation is a phase transition with a well-defined density-temperature phase diagram. The measured phase boundary agrees well with the predictions of basic quantum gas theory.
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Early works assessed thermality in terms of the momentum distribution approaching or not a Bose-Einstein distribution at a well-defined temperature and chemical potential, while recent works have highlighted the need to establish thermalization in terms of rigorous fluctuation-dissipation relations and frequency-dependent observables.
“While early works have assessed thermality in terms of the momentum distribution approaching or not a Bose-Einstein distribution at a well defined temperaturefoot_3 and chemical potential [119,120], recent works have highlighted the need to establish thermalization in terms of rigorous fluctuation-dissipation relations and frequency-dependent observables [121].”
From How to exploit driving and dissipation to stabilize and manipulate quantum many-body states (2025) · cites this paper as [120]
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Cites
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Kéna-Cohen, S., & Forrest, S. R. (2010) · Nature Photonics · doi:10.1038/nphoton.2010.86 · Cited by 942 · see citing works
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How to exploit driving and dissipation to stabilize and manipulate quantum many-body states
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“In addition to the optimized planar microcavity devices to study, e.g., quasi-equilibrium Bose-Einstein condensation effects in polariton fluids [31, 32], such a strategy is implicitly undertaken in experiments addressing the many-body physics of microwave photons in superconductor-based…”
- Authors
- Sun, Y., Wen, P., Yoon, Y., Liu, G., Steger, M., Pfeiffer, L. N., West, K., Snoke, D. W., & Nelson, K. A.
- Affiliations
- Massachusetts Institute of Technology (US)
- University of Pittsburgh (US)
- Princeton University (US)
- ORCID
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2017-01-05
- Volume
- 118
- Issue
- 1
- Pages
- 016602-016602
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2237050955
- Cited by
- 223
- References
- 2
- Citations by year
- 2026: 13 · 2025: 16 · 2024: 16 · 2023: 18 · 2022: 17 · 2021: 25 · 2020: 20 · 2019: 30 · 2018: 44 · 2017: 23 · 2016: 1
- FWCI
- 15.69
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- DSpace@MIT (Massachusetts Institute of Technology) (submittedVersion, cc-by-nc)
- arXiv (Cornell University)
- Funders
- U.S. Department of Energy
- Office of Science
- Basic Energy Sciences (DE-SC0001088)
- National Science Foundation (PHY-1205762, DMR-1104383, DMR-1420541)
- Gordon and Betty Moore Foundation (GBMF4420)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Strong Light-Matter Interactions
- Physical Sciences › Engineering › Biomedical Engineering › Plasmonic and Surface Plasmon Research
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Mechanical and Optical Resonators
- Keywords
- Bose-Einstein condensation, microcavity polaritons, thermal equilibrium, polariton lifetime, non-equilibrium condensation, phase transitions, high-Q microcavities, superfluidity
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