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Many-Molecule Reaction Triggered by a Single Photon in Polaritonic Chemistry
Open accessAbstract
The second law of photochemistry states that, in most cases, no more than one molecule is activated for an excited-state reaction for each photon absorbed by a collection of molecules. In this Letter, we demonstrate that it is possible to trigger a many-molecule reaction using only one photon by strongly coupling the molecular ensemble to a confined light mode. The collective nature of the resulting hybrid states of the system (the so-called polaritons) leads to the formation of a polaritonic "supermolecule" involving the degrees of freedom of all molecules, opening a reaction path on which all involved molecules undergo a chemical transformation. We theoretically investigate the system conditions for this effect to take place and be enhanced.
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Cites
Nonlinear Interactions in an Organic Polariton Condensate
Daskalakis, K. S., Maier, S. A., Murray, R., & Kéna-Cohen, S. (2014) · Nature Materials · doi:10.1038/nmat3874 · Cited by 484
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Metadata
- Authors
- Galego, J., Garcia-Vidal, F. J., & Feist, J.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2017-09-27
- Volume
- 119
- Issue
- 13
- Pages
- 136001-136001
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2608748366
- Cited by
- 165
- References
- 1
- FWCI
- 9.31
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Galego, J., Garcia-Vidal, F. J., & Feist, J. (2017). Many-Molecule Reaction Triggered by a Single Photon in Polaritonic Chemistry. Physical Review Letters. https://doi.org/10.1103/physrevlett.119.136001
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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