Atomic-Level Viscosity Distribution in the Hydration Layer
Open accessAbstract
The viscosity of solvation structures is crucial for the development of energy-efficient biofunctional and electrochemical devices. Elucidating their subnanoscale distributions can cause the formation of a sustainable energy society. Here, we visualize the site-specific three-dimensional damping distribution on a CaCO_{3} surface composed of binary ion species using ultra-low-noise frequency modulation atomic force microscopy. With the support from molecular dynamics simulation, we found a strikingly large damping at the calcium sites, which demonstrates the capability of this methodology to visualize atomic-scale viscosity in the hydration layers. Our finding will expedite the evolutions of various functional devices.
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Flagged first, then by citations
Research works printed but not linked: 2
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Sorted by citations
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- Authors
- Umeda, K., Kobayashi, K., Minato, T., & Yamada, H.
- Affiliations
- Kanazawa University (JP)
- Kyoto University (JP)
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2019-03-21
- Volume
- 122
- Issue
- 11
- Pages
- 116001-116001
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2922943116
- Cited by
- 37
- References
- 32
- Citations by year
- 2026: 3 · 2025: 4 · 2024: 7 · 2023: 3 · 2022: 9 · 2021: 5 · 2020: 4 · 2019: 2
- FWCI
- 2.31
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- Institutional Repositories DataBase (IRDB) (submittedVersion)
- Kyoto University Research Information Repository (Kyoto University) (submittedVersion)
- Funders
- Japan Society for the Promotion of Science (24221008, 25286057, 15K17467, 16J01165)
- Murata Science Foundation
- Foundation Advanced Technology Institute
- Nanotech Career-up Alliance
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Force Microscopy Techniques and Applications
- Physical Sciences › Chemistry › Physical and Theoretical Chemistry › Electrostatics and Colloid Interactions
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Spectroscopy and Quantum Chemical Studies
- Keywords
- hydration shell, solvation structure, frequency modulation atomic force microscopy, calcium binding sites, molecular dynamics simulation
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