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Layering Transitions and Dynamics of Confined Liquid Films
Abstract
Using grand-canonical molecular dynamics simulations and free energy calculations of spherical molecular confined films, we investigate the internal energy and entropic origins of density layering and solvation force oscillations. We show that these properties, as well as diffusion and rheological characteristics of such films, depend on interfacial commensurability, with commensurate films exhibiting abrupt solidification for relatively thick, 5 or 6 layer, films.
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Cites
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Cited by
Computer Simulation of Liquids
Allen, M. P., & Tildesley, D. J. (2017) · doi:10.1093/oso/9780198803195.001.0001 · Cited by 20,945
The nonlinear nature of friction
Urbakh, M., Klafter, J., Gourdon, D., & Israelachvili, J. (2004) · Nature · doi:10.1038/nature02750 · Cited by 696
Fluidity of water confined to subnanometre films
Raviv, U., Laurat, P., & Klein, J. (2001) · Nature · doi:10.1038/35092523 · Cited by 660
Confinement effects on freezing and melting
Christenson, H. K. (2001) · Journal of Physics: Condensed Matter · doi:10.1088/0953-8984/13/11/201 · Cited by 567
Klein, J., & Kumacheva, E. (1998) · The Journal of Chemical Physics · doi:10.1063/1.476114 · Cited by 496
Metadata
- Authors
- Gao, J., Luedtke, W. D., & Landman, U.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 1997-07-28
- Volume
- 79
- Issue
- 4
- Pages
- 705-708
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W1976833925
- Cited by
- 364
- References
- 1
- FWCI
- 13.40
- Type
- journal article
- Language
- en
- Open access
- closed
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- Gao, J., Luedtke, W. D., & Landman, U. (1997). Layering Transitions and Dynamics of Confined Liquid Films. Physical Review Letters. https://doi.org/10.1103/physrevlett.79.705
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
