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Observation of Hot-Electron Pressure in the Vibration Dynamics of Metal Nanoparticles
Abstract
We investigate the vibration dynamics of ellipsoidal silver nanoparticles, using time-resolved optical pump-probe spectroscopy. When excited with femtosecond laser pulses, the particles execute anisotropic shape oscillations. We show that these vibrations are triggered by the thermal expansion of the optically heated particles. The time dependence of the vibrations indicates that this expansion is caused by two mechanisms: The lattice anharmonicity and the extremely large pressure of the hot conduction electrons.
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Citations
Cited by
Ghosh, S. K., & Pal, T. (2007) · Chemical Reviews · doi:10.1021/cr0680282 · Cited by 2,782
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Characterization of nanostructured metal films by picosecond acoustics and interferometry
O’Hara, K. E., Hu, X., & Cahill, D. G. (2001) · Journal of Applied Physics · doi:10.1063/1.1406543 · Cited by 95
Probing the Gold Nanorod−Ligand−Solvent Interface by Plasmonic Absorption and Thermal Decay
Schmidt, A. J., Alper, J. D., Chiesa, M., Chen, G., Das, S. K., & Hamad-Schifferli, K. (2008) · The Journal of Physical Chemistry C · doi:10.1021/jp8051888 · Cited by 91
Momentum Distribution of Electrons Emitted from Resonantly Excited Individual Gold Nanorods
Lehr, M., Foerster, B., Schmitt, M., Krüger, K., Sönnichsen, C., Schönhense, G., & Elmers, H.-J. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b02434 · Cited by 37
Metadata
- Authors
- Perner, M., Gresillon, S., März, J., von Plessen, G., Feldmann, J., Porstendorfer, J., Berg, K.-J., & Berg, G.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2000-07-24
- Volume
- 85
- Issue
- 4
- Pages
- 792-795
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2039638265
- Cited by
- 226
- References
- 0
- FWCI
- 5.34
- Type
- journal article
- Language
- en
- Open access
- closed
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- Perner, M., Gresillon, S., März, J., von Plessen, G., Feldmann, J., Porstendorfer, J., Berg, K.-J., & Berg, G. (2000). Observation of Hot-Electron Pressure in the Vibration Dynamics of Metal Nanoparticles. Physical Review Letters. https://doi.org/10.1103/physrevlett.85.792
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