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Transform-Limited Pulses Are Not Optimal for Resonant Multiphoton Transitions
Open accessAbstract
Maximizing nonlinear light-matter interactions is a primary motive for compressing laser pulses to achieve ultrashort transform limited pulses. Here we show how, by appropriately shaping the pulses, resonant multiphoton transitions can be enhanced significantly beyond the level achieved by maximizing the pulse's peak intensity. We demonstrate the counterintuitive nature of this effect with an experiment in a resonant two-photon absorption, in which, by selectively removing certain spectral bands, the peak intensity of the pulse is reduced by a factor of 40, yet the absorption rate is doubled. Furthermore, by suitably designing the spectral phase of the pulse, we increase the absorption rate by a factor of 7.
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Cites
Shaped-pulse optimization of coherent emission of high-harmonic soft X-rays
Bartels, R., Backus, S., Zeek, E., Misoguti, L., Vdovin, G., Christov, I. P., Murnane, M. M., & Kapteyn, H. C. (2000) · Nature · doi:10.1038/35018029 · Cited by 713
Cited by
Principles of two-photon excitation microscopy and its applications to neuroscience
Svoboda, K., & Yasuda, R. (2006) · Neuron · doi:10.1016/j.neuron.2006.05.019 · Cited by 1,027
Colloquium: Coherently controlled adiabatic passage
Král, P., Thanopulos, I., & Shapiro, M. (2007) · Reviews of Modern Physics · doi:10.1103/revmodphys.79.53 · Cited by 444
United Time-Frequency Spectroscopy for Dynamics and Global Structure
Marian, A., Stowe, M. C., Lawall, J. R., Felinto, D., & Ye, J. (2004) · Science · doi:10.1126/science.1105660 · Cited by 294
Bigourd, D., Chatel, B., Schleich, W. P., & Girard, B. (2008) · Physical Review Letters · doi:10.1103/physrevlett.100.030202 · Cited by 84
Metadata
- Authors
- Dudovich, N., Dayan, B., Gallagher Faeder, S. M., & Silberberg, Y.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2001-01-01
- Volume
- 86
- Issue
- 1
- Pages
- 47-50
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2055741917
- Cited by
- 279
- References
- 1
- FWCI
- 8.49
- Type
- journal article
- Language
- en
- Open access
- green
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- Dudovich, N., Dayan, B., Gallagher Faeder, S. M., & Silberberg, Y. (2001). Transform-Limited Pulses Are Not Optimal for Resonant Multiphoton Transitions. Physical Review Letters. https://doi.org/10.1103/physrevlett.86.47
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