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Strong Exciton-Photon Coupling and Exciton Hybridization in a Thermally Evaporated Polycrystalline Film of an Organic Small Molecule
Abstract
We demonstrate strong exciton-photon coupling in an optical microcavity containing a thermally evaporated polycrystalline organic thin film. Microcavity polaritons result from coupling between the 0-0 excitonic transition of 3,4,7,8 napthalenetetracarboxylic dianhydride and a cavity photon. For thicker films, the 0-1 transition also couples to the cavity mode, as vibronic relaxation is overcome by the short Rabi period for strong coupling. To our knowledge, this is the first report of strong coupling between a cavity photon and multiple vibronic transitions in a single material, made possible by the pronounced vibronic absorption features characteristic of crystalline organic materials.
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Hutchison, J. A., Schwartz, T., Genet, C., Devaux, E., & Ebbesen, T. W. (2012) · Angewandte Chemie International Edition · doi:10.1002/anie.201107033 · Cited by 932
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Plumhof, J. D., Stöferle, T., Mai, L., Scherf, U., & Mahrt, R. F. (2014) · Nature Materials · doi:10.1038/nmat3825 · Cited by 745
Reversible Switching of Ultrastrong Light-Molecule Coupling
Schwartz, T., Hutchison, J. A., Genet, C., & Ebbesen, T. W. (2011) · Physical Review Letters · doi:10.1103/physrevlett.106.196405 · Cited by 658
Polariton-Mediated Energy Transfer between Organic Dyes in a Strongly Coupled Optical Microcavity
Coles, D. M., Somaschi, N., Michetti, P., Clark, C., Lagoudakis, P. G., Savvidis, P. G., & Lidzey, D. G. (2014) · Nature Materials · doi:10.1038/nmat3950 · Cited by 507
Metadata
- Authors
- Holmes, R. J., & Forrest, S. R.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2004-10-28
- Volume
- 93
- Issue
- 18
- Pages
- 186404-186404
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2052906153
- Cited by
- 166
- References
- 0
- FWCI
- 3.48
- Type
- journal article
- Language
- en
- Open access
- closed
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- Holmes, R. J., & Forrest, S. R. (2004). Strong Exciton-Photon Coupling and Exciton Hybridization in a Thermally Evaporated Polycrystalline Film of an Organic Small Molecule. Physical Review Letters. https://doi.org/10.1103/physrevlett.93.186404
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