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Superaerophilic/superaerophobic cooperative electrode for efficient hydrogen evolution reaction via enhanced mass transfer
Open accessAbstract
Hydrogen evolution reaction (HER), as an effective method to produce green hydrogen, is greatly impeded by inefficient mass transfer, i.e., bubble adhesion on electrode, bubble dispersion in the vicinity of electrode, and poor dissolved H 2 diffusion, which results in blocked electrocatalytic area and large H 2 concentration overpotential. Here, we report a superaerophilic/superaerophobic (SAL/SAB) cooperative electrode to efficiently promote bubble transfer by asymmetric Laplace pressure and accelerate dissolved H 2 diffusion through reducing diffusion distance. Benefiting from the enhanced mass transfer, the overpotential for the SAL/SAB cooperative electrode at −10 mA cm −2 is only −19 mV, compared to −61 mV on the flat Pt electrode. By optimizing H 2 SO 4 concentration, the SAL/SAB cooperative electrode can achieve ultrahigh current density (−1867 mA cm −2 ) at an overpotential of −500 mV. We can envision that the SAL/SAB cooperative strategy is an effective method to improve HER efficiency and stimulate the understanding of various gas-involved processes.
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“Furthermore, introducing aerophobic/aerophilic patterned designs [176, 177] can further modulate bubble migration trajectories.”
From Advances in Surface/Interface Engineering of Under-Water Superaerophobic Electrodes for Hydrogen Evolution Reaction by Manipulating of Bubbles (2026) · cites this paper as [176]
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Metadata
- Authors
- Zhang, C., Xu, Z., Han, N., Tian, Y., Kallio, T., Yu, C., & Jiang, L.
- Affiliations
- Chinese Academy of Sciences (CN)
- Beihang University (CN)
- Aalto University (FI)
- Corresponding author
- Yu, Cunming
- Jiang, Lei
- Venue
- Science Advances
- Published
- 2023-01-20
- Volume
- 9
- Issue
- 3
- Pages
- eadd6978-eadd6978
- ISSN
- 2375-2548 (ISSN-L)
- PMC
- PMC9848275
- OpenAlex
- W4317254717
- Cited by
- 230
- References
- 66
- Citations by year
- 2026: 70 · 2025: 66 · 2024: 63 · 2023: 31
- FWCI
- 10.99
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- cc-by-nc
- Locations
- Science Advances (publishedVersion, cc-by-nc)
- PubMed Central (publishedVersion, cc-by-nc)
- PubMed (publishedVersion)
- Aaltodoc (Aalto University) (submittedVersion, cc-by-nc)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Surfaces, Coatings and Films › Surface Modification and Superhydrophobicity
- Physical Sciences › Chemical Engineering › Filtration and Separation › Minerals Flotation and Separation Techniques
- Keywords
- hydrogen evolution reaction, superaerophobic surfaces, bubble adhesion, bubble dispersion, Laplace pressure, hydrogen diffusion, mass transfer enhancement, green hydrogen production, electrocatalysis, sulfuric acid electrolyte
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