Cited by 1,037Catalytic Processes in Materials ScienceMesoporous Materials and CatalysisMetal-Organic Frameworks: Synthesis and Applications

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Catalytic nanoarchitectures—The importance of nothing and the unimportance of periodicity

Rolison, Debra R.·2003·Science

DOI 10.1126/science.1082332

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Abstract

Heterogeneous catalysis has always been an inherently nanoscopic phenomenon with important technological and societal consequences for energy conversion and the production of chemicals. New opportunities for improved performance arise when the multifunctionality inherent in catalytic processes, including molecular transport of reactants and products, is rethought in light of architectures designed and fabricated from the appropriate nanoscale building blocks, including the use of "nothing" (void space) and deliberate disorder as design components. Architectures with all of the appropriate electrochemical and catalytic requirements, including large surface areas readily accessible to molecules, may now be assembled on the benchtop. Designing catalytic nanoarchitectures that depart from the hegemony of periodicity and order offers the promise of even higher activity.

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Authors: Rolison, D. R.
Affiliations: United States Naval Research Laboratory (US)
Corresponding author: Rolison, Debra R.
ORCID: Rolison, Debra R.
Venue: Science
Publisher: American Association for the Advancement of Science (AAAS)
Published: 2003-03-14
Volume: 299
Issue: 5613
Pages: 1698-1701
ISSN: 0036-8075 (ISSN-L)
1095-9203
DOI: 10.1126/science.1082332
OpenAlex: W1965751645
Cited by: 1,037
References: 35
Citations by year: 2026: 10 · 2025: 16 · 2024: 13 · 2023: 19 · 2022: 22 · 2021: 22 · 2020: 19 · 2019: 24 · 2018: 45 · 2017: 53 · 2016: 63 · 2015: 55 · 2014: 53 · 2013: 67 · 2012: 73
FWCI: 33.53
Type: journal article
Language: en
Open access: closed
Locations: Science (publishedVersion)
PubMed (publishedVersion)
Topics: Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
Physical Sciences › Materials Science › Materials Chemistry › Mesoporous Materials and Catalysis
Physical Sciences › Chemistry › Inorganic Chemistry › Metal-Organic Frameworks: Synthesis and Applications
Keywords: heterogeneous catalysis, voids, disorder, aperiodic structures, molecular transport, surface area, electrocatalysis, nanoscale building blocks, catalyst design

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Catalytic nanoarchitectures—The importance of nothing and the unimportance of periodicity

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