The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Selective conversion of syngas to light olefins
Abstract
Small olefins from syngas: The conversion of coal or natural gas to liquid fuels or chemicals often proceeds through the production of CO and H 2 . This mixture, known as syngas, is then converted to hydrocarbons with Fischer-Tropsch catalysts. For the light olefins (ethylene to butylenes) needed for chemical and polymer synthesis, conventional catalysts are mechanistically limited to <60% conversion and deactivate through carbon buildup. Jiao et al. developed a bifunctional catalyst that achieves higher conversions and avoids deactivation (see the Perspective by de Jong). A zinc-chromium oxide creates ketene intermediates that are then coupled over a zeolite. Science , this issue p. 1065 , see also p. 1030
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Cites
Generalized Gradient Approximation Made Simple
Perdew, J. P., Burke, K., & Ernzerhof, M. (1996) · Physical Review Letters · doi:10.1103/physrevlett.77.3865 · Cited by 215,824
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Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Direct conversion of CO2 into liquid fuels with high selectivity over a bifunctional catalyst
Gao, P., Li, S., Bu, X., Dang, S., Liu, Z., Wang, H., Zhong, L., Qiu, M., Yang, C., Cai, J., et al. (2017) · Nature Chemistry · doi:10.1038/nchem.2794 · Cited by 1,122
Cobalt carbide nanoprisms for direct production of lower olefins from syngas
Zhong, L., Yu, F., An, Y., Zhao, Y., Sun, Y., Li, Z., Lin, T., Lin, Y., Qi, X., Dai, Y., et al. (2016) · Nature · doi:10.1038/nature19786 · Cited by 874
Technical photosynthesis involving CO2 electrolysis and fermentation
Haas, T., Krause, R., Weber, R., Demler, M., & Schmid, G. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0005-1 · Cited by 649
Cheng, K., Zhou, W., Kang, J., He, S., Shi, S., Zhang, Q., Pan, Y., Wen, W., & Wang, Y. (2017) · Chem · doi:10.1016/j.chempr.2017.05.007 · Cited by 533
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Metadata
- Authors
- Jiao, F., Li, J., Pan, X., Xiao, J., Li, H., Ma, H., Wei, M., Pan, Y., Zhou, Z., Li, M., Miao, S., Li, J., Zhu, Y., Xiao, D., He, T., Yang, J., Qi, F., Fu, Q., & Bao, X.
- Venue
- Science
- Published
- 2016-03-04
- Volume
- 351
- Issue
- 6277
- Pages
- 1065-1068
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2323504704
- Cited by
- 1,521
- References
- 1
- FWCI
- 40.34
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Jiao, F., Li, J., Pan, X., Xiao, J., Li, H., Ma, H., Wei, M., Pan, Y., Zhou, Z., Li, M., Miao, S., Li, J., Zhu, Y., Xiao, D., He, T., Yang, J., Qi, F., Fu, Q., & Bao, X. (2016). Selective conversion of syngas to light olefins. Science. https://doi.org/10.1126/science.aaf1835
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