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Nanogoethite is the dominant reactive oxyhydroxide phase in lake and marine sediments
Open accessAbstract
Iron oxides affect many elemental cycles in aquatic sediments via numerous redox reactions and their large sorption capacities for phosphate and trace elements. The reactive ferric oxides and oxyhydroxides are usually quantified by operationally defined selective chemical extractions that are not mineral specific. We have used cryogenic 57Fe Mössbauer spectroscopy to show that the reactive iron oxyhydroxide phase in a large variety of lacustrine and marine environments is nanophase goethite (α-FeOOH), rather than the assumed surface-complex–stabilized, two-line ferrihydrite and accompanying mixture of clay and oxyhydroxide Fe-bearing phases. This result implies that the kinetic and stability parameters of the type of nanogoethite that we observe to be present in sediments should be first determined and then used in models of early diagenesis. The identity and characteristics of the reactive phase will also set constraints on the mechanisms of its authigenesis.
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Cited by
Rickard, D., & Luther, G. W. (2007) · Chemical Reviews · doi:10.1021/cr0503658 · Cited by 1,599
Preservation of organic matter in sediments promoted by iron
Lalonde, K., Mucci, A., Ouellet, A., & Gélinas, Y. (2012) · Nature · doi:10.1038/nature10855 · Cited by 1,509
Natural, incidental, and engineered nanomaterials and their impacts on the Earth system
Hochella, M. F., Mogk, D. W., Ranville, J., Allen, I. C., Luther, G. W., Marr, L. C., McGrail, B. P., Murayama, M., Qafoku, N. P., Rosso, K. M., et al. (2019) · Science · doi:10.1126/science.aau8299 · Cited by 833
Nanotechnology and in Situ Remediation: A Review of the Benefits and Potential Risks
Karn, B., Kuiken, T., & Otto, M. (2009) · Environmental Health Perspectives · doi:10.1289/ehp.0900793 · Cited by 721
Rickard, D., & Morse, J. W. (2005) · Marine Chemistry · doi:10.1016/j.marchem.2005.08.004 · Cited by 632
Metadata
- Authors
- van der Zee, C., Roberts, D. R., Rancourt, D. G., & Slomp, C. P.
- Venue
- Geology
- Publisher
- Geological Society of America
- Published
- 2003
- Volume
- 31
- Issue
- 11
- Pages
- 993
- ISSN
- 0091-7613 (ISSN-L)
- OpenAlex
- W2134307060
- Cited by
- 314
- References
- 2
- FWCI
- 13.62
- Type
- journal article
- Language
- en
- Open access
- green
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- van der Zee, C., Roberts, D. R., Rancourt, D. G., & Slomp, C. P. (2003). Nanogoethite is the dominant reactive oxyhydroxide phase in lake and marine sediments. Geology. https://doi.org/10.1130/g19924.1
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