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ULTRAFAST CHEMISTRY: Using Time-Resolved Vibrational Spectroscopy for Interrogation of Structural Dynamics
Abstract
▪ Abstract Time-resolved infrared (IR) and Raman spectroscopy elucidates molecular structure evolution during ultrafast chemical reactions. Following vibrational marker modes in real time provides direct insight into the structural dynamics, as is evidenced in studies on intramolecular hydrogen transfer, bimolecular proton transfer, electron transfer, hydrogen bonding during solvation dynamics, bond fission in organometallic compounds and heme proteins, cis-trans isomerization in retinal proteins, and transformations in photochromic switch pairs. Femtosecond IR spectroscopy monitors the site-specific interactions in hydrogen bonds. Conversion between excited electronic states can be followed for intramolecular electron transfer by inspection of the fingerprint IR- or Raman-active vibrations in conjunction with quantum chemical calculations. Excess internal vibrational energy, generated either by optical excitation or by internal conversion from the electronic excited state to the ground state, is observable through transient frequency shifts of IR-active vibrations and through nonequilibrium populations as deduced by Raman resonances.
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Grabowski, Z. R., Rotkiewicz, K., & Rettig, W. (2003) · Chemical Reviews · doi:10.1021/cr940745l · Cited by 3,714
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Middleton, C. T., de La Harpe, K., Su, C., Law, Y. K., Crespo-Hernández, C. E., & Kohler, B. (2009) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.59.032607.093719 · Cited by 827
Femtosecond Stimulated Raman Spectroscopy
Kukura, P., McCamant, D. W., & Mathies, R. A. (2007) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.58.032806.104456 · Cited by 632
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Metadata
- Authors
- Nibbering, E. T. J., Fidder, H., & Pines, E.
- Venue
- Annual Review of Physical Chemistry
- Publisher
- Annual Reviews
- Published
- 2005-05-05
- Volume
- 56
- Issue
- 1
- Pages
- 337-367
- ISSN
- 0066-426X (ISSN-L)
- 1545-1593
- OpenAlex
- W2169983477
- Cited by
- 326
- References
- 1
- FWCI
- 0.89
- Type
- journal article
- Language
- en
- Open access
- closed
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- Nibbering, E. T. J., Fidder, H., & Pines, E. (2005). ULTRAFAST CHEMISTRY: Using Time-Resolved Vibrational Spectroscopy for Interrogation of Structural Dynamics. Annual Review of Physical Chemistry. https://doi.org/10.1146/annurev.physchem.56.092503.141314
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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