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Femtosecond Stimulated Raman Spectroscopy
Abstract
Femtosecond stimulated Raman spectroscopy (FSRS) is a new ultrafast spectroscopic technique that provides vibrational structural information with high temporal (50-fs) and spectral (10-cm−1) resolution. As a result of these unique capabilities, FSRS studies of chemical and biochemical reaction dynamics are expected to grow rapidly, giving previously unattainable insight into the structural dynamics of reactively evolving systems with atomic spatial and femtosecond temporal resolution. This review discusses the experimental and theoretical concepts behind FSRS, with an emphasis on the origins of its unique temporal and spectral capabilities. We illustrate these capabilities with vibrational studies of ultrafast electronic dynamics, as well as the direct structural observation of nonstationary vibrational wave-packet motion in small molecules and in complex biochemical reaction dynamics.
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Citations
Cites
Two-Dimensional Femtosecond Spectroscopy
Jonas, D. M. (2003) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.54.011002.103907 · Cited by 1,198
The First Step in Vision: Femtosecond Isomerization of Rhodopsin
Schoenlein, R. W., Peteanu, L. A., Mathies, R. A., & Shank, C. V. (1991) · Science · doi:10.1126/science.1925597 · Cited by 892
Self-citation
Cited by
Chemical mapping of a single molecule by plasmon-enhanced Raman scattering
Zhang, R., Zhang, Y., Dong, Z. C., Jiang, S., Zhang, C., Chen, L. G., Zhang, L., Liao, Y., Aizpurua, J., Luo, Y., et al. (2013) · Nature · doi:10.1038/nature12151 · Cited by 1,770
Biological imaging of chemical bonds by stimulated Raman scattering microscopy
Hu, F., Shi, L., & Min, W. (2019) · Nature Methods · doi:10.1038/s41592-019-0538-0 · Cited by 392
Nonlinear optical signals and spectroscopy with quantum light
Dorfman, K. E., Schlawin, F., & Mukamel, S. (2016) · Reviews of Modern Physics · doi:10.1103/revmodphys.88.045008 · Cited by 361
Stimulated Raman Scattering: From Bulk to Nano
Prince, R. C., Frontiera, R. R., & Potma, E. O. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00545 · Cited by 350
Non-classicality of the molecular vibrations assisting exciton energy transfer at room temperature
O’Reilly, E. J., & Olaya-Castro, A. (2014) · Nature Communications · doi:10.1038/ncomms4012 · Cited by 230
Metadata
- Authors
- Kukura, P., McCamant, D. W., & Mathies, R. A.
- Venue
- Annual Review of Physical Chemistry
- Publisher
- Annual Reviews
- Published
- 2007-05-01
- Volume
- 58
- Issue
- 1
- Pages
- 461-488
- ISSN
- 0066-426X (ISSN-L)
- 1545-1593
- OpenAlex
- W2910581328
- Cited by
- 632
- References
- 2
- FWCI
- 1.27
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kukura, P., McCamant, D. W., & Mathies, R. A. (2007). Femtosecond Stimulated Raman Spectroscopy. Annual Review of Physical Chemistry. https://doi.org/10.1146/annurev.physchem.58.032806.104456
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