Cited by 353Fuel Cells and Related MaterialsAdvancements in Solid Oxide Fuel CellsElectrocatalysts for Energy Conversion

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Water Management in PEM Fuel Cells

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Berg, Peter, Promislow, Keith, St. Pierre, Jean, Stumper, Jürgen, Wetton, Brian·2004·Journal of The Electrochemical Society

DOI 10.1149/1.1641033

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Abstract

A simplified model for water management in a polymer electrolyte membrane (PEM) fuel cell operating under prescribed current with iso-potential plates is presented. The consumption of gases in the flow field channels, coupled to the electric potential and water content in the polymer membrane, is modeled in a two-dimensional slice from inlet to outlet and through the membrane. Both co- and counter-flowing air and fuel streams are considered, with attention paid to sensitivity of along-the-channel current density to inlet humidities, gas stream composition, and fuel and oxygen stoichiometries. The parameters describing the nonequilibrium kinetics of the membrane/catalyst interface are found to be fundamental to accurate fuel cell modeling. A new parameter which models nonequilibrium membrane water uptake rates is introduced. Four parameters, the exchange current, a membrane water transfer coefficient, an effective oxygen diffusivity, and an average membrane resistance, are fit to a subset of data and then held constant in subsequent runs which compare polarization curves, current density and membrane hydration distributions, water transfer, and stoichiometric sensitivity to the balance of the experimental data. © 2004 The Electrochemical Society. All rights reserved.

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Authors: Berg, P., Promislow, K., St. Pierre, J., Stumper, J., & Wetton, B.
Affiliations: Simon Fraser University (CA)
University of British Columbia (CA)
ORCID: Berg, Peter
Promislow, Keith
Wetton, Brian
Venue: Journal of The Electrochemical Society
Publisher: The Electrochemical Society
Published: 2004
Volume: 151
Issue: 3
Pages: A341
ISSN: 0013-4651 (ISSN-L)
DOI: 10.1149/1.1641033
OpenAlex: W2103992671
Cited by: 353
References: 29
Citations by year: 2026: 5 · 2025: 10 · 2024: 9 · 2023: 11 · 2022: 7 · 2021: 7 · 2020: 8 · 2019: 10 · 2018: 6 · 2017: 9 · 2016: 8 · 2015: 7 · 2014: 11 · 2013: 13 · 2012: 27
FWCI: 32.23
Type: journal article
Language: en
Open access: bronze
doi.org
Locations: Journal of The Electrochemical Society (publishedVersion)
Funders: Ballard Power Systems
Simon Fraser University
Mitacs
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
Physical Sciences › Materials Science › Materials Chemistry › Advancements in Solid Oxide Fuel Cells
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Keywords: proton exchange membrane fuel cells, water management (fuel cells), membrane hydration, water transport, nonequilibrium kinetics, stoichiometry, current density distribution, polarization curves, oxygen diffusion coefficient, membrane resistance

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Water Management in PEM Fuel Cells

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