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Lithium Sulfur Battery: Oxidation/Reduction Mechanisms of Polysulfides in THF Solutions
Open accessAbstract
The redox processes of at a glassy carbon electrode in THF was studied by programmed cyclic voltammetry in the range of +1300 to −2000 mV ( vs. polysulfide reference electrode) at sweep rates of 2–200 mV/s. One anodic and up to three cathodic peaks were detected. The anodic peak seems to result from the oxidation of all PS's through the same intermediate to elemental sulfur. The first cathodic peak is caused by the reduction of all PS to in a diffusion controlled reaction. The second reduction peak most likely arises from the reduction of to . This is apparently preceded by a chemical step. The third reduction peak is caused by the reduction of to or S 2− or a mixture of both in a diffusion‐controlled reaction. The high Tafel slope of the third peak apparently results from passivation of the electrode by the precipitation of and .
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Cited by
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Wei Seh, Z., Li, W., Cha, J. J., Zheng, G., Yang, Y., McDowell, M. T., Hsu, P.-C., & Cui, Y. (2013) · Nature Communications · doi:10.1038/ncomms2327 · Cited by 2,107
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Liang, J., Sun, Z.-H., Li, F., & Cheng, H.-M. (2016) · Energy Storage Materials · doi:10.1016/j.ensm.2015.09.007 · Cited by 593
Electrochemical performance of lithium/sulfur cells with three different polymer electrolytes
Marmorstein, D., Yu, T. H., Striebel, K. A., McLarnon, F. R., Hou, J., & Cairns, E. J. (2000) · Journal of Power Sources · doi:10.1016/s0378-7753(00)00432-8 · Cited by 451
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Metadata
- Authors
- Yamin, H., Gorenshtein, A., Penciner, J., Sternberg, Y., & Peled, E.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1988-05-01
- Volume
- 135
- Issue
- 5
- Pages
- 1045-1048
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W1620090426
- Cited by
- 471
- References
- 0
- FWCI
- 0.48
- Type
- journal article
- Language
- en
- Open access
- bronze
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- CoChat. (2026). Citation check: Lithium Sulfur Battery: Oxidation/Reduction Mechanisms of Polysulfides in THF Solutions. https://app.cochat.ai/papers/10.1149/1.2095868
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- Yamin, H., Gorenshtein, A., Penciner, J., Sternberg, Y., & Peled, E. (1988). Lithium Sulfur Battery: Oxidation/Reduction Mechanisms of Polysulfides in THF Solutions. Journal of The Electrochemical Society. https://doi.org/10.1149/1.2095868
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
