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Effect of Electrolyte Composition on Lithium Dendrite Growth
Open accessAbstract
Lithium deposition is observed in situ using a microfluidic test cell. The microfluidic device rapidly sets up a steady concentration gradient and minimizes ohmic potential loss, minimizes electrolyte usage, and shows good repeatability. Dendrite growth is observed at different current densities for electrolytes containing lithium hexafluorophosphate or lithium bis(trifluoromethane sulfonyl) imide (LiTFSI) in mixtures of propylene carbonate (PC) and dimethyl carbonate. Dendrites are formed at shorter times in electrolytes containing LiTFSI and high amounts of PC. The time to first observed dendrites increases linearly (for all electrolyte compositions) with a resistance given by the Tafel slope of the lithium reduction polarization curve.
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Cites
Advanced Model for Solid Electrolyte Interphase Electrodes in Liquid and Polymer Electrolytes
Peled, E., Golodnitsky, D., & Ardel, G. (1997) · Journal of The Electrochemical Society · doi:10.1149/1.1837858 · Cited by 1,205
Cited by
An, S. J., Li, J., Daniel, C., Mohanty, D., Nagpure, S., & Wood, D. L. (2016) · Carbon · doi:10.1016/j.carbon.2016.04.008 · Cited by 2,121
Interconnected hollow carbon nanospheres for stable lithium metal anodes
Zheng, G., Lee, S. W., Liang, Z., Lee, H.-W., Yan, K., Yao, H., Wang, H., Li, W., Chu, S., & Cui, Y. (2014) · Nature Nanotechnology · doi:10.1038/nnano.2014.152 · Cited by 1,764
Lithium-ion battery fast charging: A review
Tomaszewska, A., Chu, Z., Feng, X., O'Kane, S., Liu, X., Chen, J., Ji, C., Endler, E., Li, R., Liu, L., et al. (2019) · eTransportation · doi:10.1016/j.etran.2019.100011 · Cited by 1,592
The synergetic effect of lithium polysulfide and lithium nitrate to prevent lithium dendrite growth
Li, W., Yao, H., Yan, K., Zheng, G., Liang, Z., Chiang, Y.-M., & Cui, Y. (2015) · Nature Communications · doi:10.1038/ncomms8436 · Cited by 1,540
Quest for Nonaqueous Multivalent Secondary Batteries: Magnesium and Beyond
Muldoon, J., Bucur, C. B., & Gregory, T. (2014) · Chemical Reviews · doi:10.1021/cr500049y · Cited by 1,376
Metadata
- Authors
- Crowther, O., & West, A. C.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2008
- Volume
- 155
- Issue
- 11
- Pages
- A806
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W2061706978
- Cited by
- 295
- References
- 1
- FWCI
- 3.29
- Type
- journal article
- Language
- en
- Open access
- bronze
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
