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Lithium–Air Batteries Using SWNT/CNF Buckypapers as Air Electrodes
Abstract
Li–air cells based on Li foil as an anode electrode, freestanding carbon nanotube/nanofiber mixed buckypaper as an air (cathode) electrode, and organic electrolyte were assembled. The air electrode was made with single-wall carbon nanotube (SWNT) and carbon nanofiber (CNF) without any binder. The discharge capacity was strongly dependent on both the discharge current density and the thickness of the air electrode. A discharge capacity as high as 2500 mAh/g was obtained for an air electrode at a thickness of 20 μ m with a discharge current density of 0.1 mA / cm 2 ; however, it was reduced to 400 mAh/g when the thickness of the air electrode was increased to 220 μ m . For a 66 μ m thick air electrode, the discharge capacity decreased from 1600 to 340 mAh/g when the discharge current density increased from 0.1 to 0.5 mA / cm 2 . The scanning electron microscope images on surfaces of the air electrode from a fully discharged cell showed that the voids at the air side were almost fully filled by the solid deposition; however, the voids at the membrane side were still wide open.
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Cited by
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Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Chen, D., Chen, C., Baiyee, Z. M., Shao, Z., & Ciucci, F. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00073 · Cited by 936
Prospective materials and applications for Li secondary batteries
Jeong, G., Kim, Y.-U., Kim, H., Kim, Y.-J., & Sohn, H.-J. (2011) · Energy & Environmental Science · doi:10.1039/c0ee00831a · Cited by 616
A review of cathode materials and structures for rechargeable lithium–air batteries
Ma, Z., Yuan, X., Li, L., Ma, Z.-F., Wilkinson, D. P., Zhang, L., & Zhang, J. (2015) · Energy & Environmental Science · doi:10.1039/c5ee00838g · Cited by 485
Shui, J.-L., Karan, N. K., Balasubramanian, M., Li, S.-Y., & Liu, D.-J. (2012) · Journal of the American Chemical Society · doi:10.1021/ja3042993 · Cited by 284
Metadata
- Authors
- Zhang, G. Q., Zheng, J. P., Liang, R., Zhang, C., Wang, B., Hendrickson, M., & Plichta, E. J.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2010
- Volume
- 157
- Issue
- 8
- Pages
- A953
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W1970125014
- Cited by
- 220
- References
- 0
- FWCI
- 17.94
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, G. Q., Zheng, J. P., Liang, R., Zhang, C., Wang, B., Hendrickson, M., & Plichta, E. J. (2010). Lithium–Air Batteries Using SWNT/CNF Buckypapers as Air Electrodes. Journal of The Electrochemical Society. https://doi.org/10.1149/1.3446852
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
