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Editors' Choice—Growth of Ambient Induced Surface Impurity Species on Layered Positive Electrode Materials and Impact on Electrochemical Performance
Open accessAbstract
Surface impurity species, most notably Li 2 CO 3 , that develop on layered oxide positive electrode materials with atmospheric aging have been reported to be highly detrimental to the subsequent electrochemical performance. LiNi 0.8 Co 0.15 Al 0.05 O 2 (NCA) was used as a model layered oxide compound to evaluate the growth and subsequent electrochemical impact of H 2 O, LiHCO 3 , LiOH and Li 2 CO 3 . Methodical high temperature annealing enabled the systematic removal of each impurity specie, thus permitting the determination of each specie's individual effect on the host material's electrochemical performance. Extensive cycling of exposed and annealed materials emphasized the cycle life degradation and capacity loss induced by each impurity, while rate capability measurements correlated the electrode impedance to the impurity species present. Based on these characterization results, this work attempts to clarify decades of ambiguity over the growth mechanisms and the electrochemical impact of the specific surface impurity species formed during powder storage in various environments.
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Cites
Ageing mechanisms in lithium-ion batteries
Vetter, J., Novák, P., Wagner, M. R., Veit, C., Möller, K.-C., Besenhard, J. O., Winter, M., Wohlfahrt-Mehrens, M., Vogler, C., & Hammouche, A. (2005) · Journal of Power Sources · doi:10.1016/j.jpowsour.2005.01.006 · Cited by 3,987
The Surface Chemistry of Lithium Electrodes in Alkyl Carbonate Solutions
Aurbach, D., Ein‐Ely, Y., & Zaban, A. (1994) · Journal of The Electrochemical Society · doi:10.1149/1.2054718 · Cited by 344
Cited by
Electrolyte Oxidation Pathways in Lithium-Ion Batteries
Rinkel, B. L. D., Hall, D. S., Temprano, I., & Grey, C. P. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c06363 · Cited by 455
Phase Behavior during Electrochemical Cycling of Ni‐Rich Cathode Materials for Li‐Ion Batteries
Xu, C., Reeves, P. J., Jacquet, Q., & Grey, C. P. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202003404 · Cited by 429
Metadata
- Authors
- Faenza, N. V., Bruce, L., Lebens-Higgins, Z. W., Plitz, I., Pereira, N., Piper, L. F. J., & Amatucci, G. G.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2017
- Volume
- 164
- Issue
- 14
- Pages
- A3727-A3741
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2774203228
- Cited by
- 205
- References
- 2
- FWCI
- 7.38
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Faenza, N. V., Bruce, L., Lebens-Higgins, Z. W., Plitz, I., Pereira, N., Piper, L. F. J., & Amatucci, G. G. (2017). Editors' Choice—Growth of Ambient Induced Surface Impurity Species on Layered Positive Electrode Materials and Impact on Electrochemical Performance. Journal of The Electrochemical Society. https://doi.org/10.1149/2.0921714jes
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