CO2 Adsorption by Functionalized Nanoporous Materials: A Review
Abstract
This review highlights the recent advances in the development of functionalized nanoporous adsorbents for CO2 capture. Three main classes of materials are taken into account: zeolites, mesoporous silicates, and metal organic frameworks (MOFs). Proper modification of the cation content of zeolites, as well as the introduction of functional groups such as amine groups into ordered mesoporous silicates and MOFs, greatly enhance the CO2 adsorptive properties of these substrates. Specifically, cation-exchanged zeolites can be currently considered the benchmark for ordered nanoporous CO2 adsorbents, finding application also on a plant scale. Amino-functionalized mesoporous silicates tend to show a high affinity toward CO2: while this could be an advantage when pushed purification is needed, it also implies that full regeneration of the adsorbent can be achieved only by putting its surface in contact with a completely CO2-free environment. On the contrary, similarly modified MOFs show higher CO2 adsorption working capacities: this potentially makes them even better candidates than their mesoporous inorganic homologues for a plant scale use. However, the persisting lack of reliable methods for the pelletization of both ordered mesoporous silicates and MOFs creates a care for further development efforts in the next future.
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Amine grafting on zeolites has gained attention in recent years for carbon capture applications.
“Amine grafing on zeolites has gained attention in the last years for carbon capture applications, although in this case the protagonists are still amine-grafted mesoporous silicas.”
From Zeolites in Adsorption Processes: State of the Art and Future Prospects (2022) · cites this paper as [158]
Adsorption is one of the most promising methods for reducing atmospheric CO2, offering excellent stability, straightforward regeneration, and effective adsorption capabilities.
“One of the most promising methods for reducing atmospheric CO2 is adsorption, which offers excellent stability, straightforward regeneration, and effective adsorption capabilities6–8.”
From Metals incorporated agricultural waste corn Cob-based biochar used as an adsorbent for CO2 capturing (2025) · cites this paper as [6]
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Klinkenberg, N., Klaiber, A., Müller, M., & Polarz, S. (2019) · Microporous and Mesoporous Materials · doi:10.1016/j.micromeso.2019.109879 · Cited by 6 · see citing works
CO2 adsorption by functionalized sorbents
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Synthesis of a New Cu-Aluminosilicate Catalyst for CO2 Capture and Conversion to Hydrocarbons
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“In studies on CO2 adsorption by PEI, a porous, inorganic material is usually impregnated with PEI [25]-[29].”
BackgroundCO2 adsorption of MSU-2 synthesized by using nonionic polyethyleneoxide (PEO)-based surfactants
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“There have been research works carried out for CO2 adsorption using mesoporous silicas including Mobil composition matter (MCM) (Beck et al., 1992), Santa Barbara Amorphous (SBA) type materials (Zhao et al., 1998) and folded sheet mesoporous material (FSM) (Gargiulo et al., 2014).”
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Fluorido-bridged iron-based metal-organic frameworks for carbon dioxide capture in humid flue gas
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- Authors
- Gargiulo, N., Pepe, F., & Caputo, D.
- Venue
- Journal of Nanoscience and Nanotechnology
- Publisher
- American Scientific Publishers
- Published
- 2014-02-01
- Volume
- 14
- Issue
- 2
- Pages
- 1811-1822
- ISSN
- 1533-4880 (ISSN-L)
- 1533-4899
- OpenAlex
- W2326306759
- Cited by
- 117
- References
- 0
- Citations by year
- 2026: 3 · 2025: 6 · 2024: 12 · 2023: 8 · 2022: 10 · 2021: 10 · 2020: 13 · 2019: 12 · 2018: 10 · 2017: 7 · 2016: 10 · 2015: 10 · 2014: 6
- FWCI
- 12.79
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Nanoscience and Nanotechnology (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Physical Sciences › Chemistry › Inorganic Chemistry › Metal-Organic Frameworks: Synthesis and Applications
- Physical Sciences › Chemistry › Inorganic Chemistry › Zeolite Catalysis and Synthesis
- Keywords
- CO2 adsorption, CO2 capture, zeolites, cation-exchanged zeolites, mesoporous silicates, metal-organic frameworks, amino-functionalized MOF, adsorbent regeneration, pelletization
- MeSH terms
- Adsorption, Carbon Dioxide, Materials Testing, Molecular Conformation, Particle Size, Surface Properties, Nanostructures, Nanopores
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