Cited by 117Carbon Dioxide Capture TechnologiesMetal-Organic Frameworks: Synthesis and ApplicationsZeolite Catalysis and Synthesis

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CO2 Adsorption by Functionalized Nanoporous Materials: A Review

Gargiulo, Nicola, Pepe, Francesco, Caputo, Domenico·2014·Journal of Nanoscience and Nanotechnology

DOI 10.1166/jnn.2014.8893

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Abstract

This review highlights the recent advances in the development of functionalized nanoporous adsorbents for CO2 capture. Three main classes of materials are taken into account: zeolites, mesoporous silicates, and metal organic frameworks (MOFs). Proper modification of the cation content of zeolites, as well as the introduction of functional groups such as amine groups into ordered mesoporous silicates and MOFs, greatly enhance the CO2 adsorptive properties of these substrates. Specifically, cation-exchanged zeolites can be currently considered the benchmark for ordered nanoporous CO2 adsorbents, finding application also on a plant scale. Amino-functionalized mesoporous silicates tend to show a high affinity toward CO2: while this could be an advantage when pushed purification is needed, it also implies that full regeneration of the adsorbent can be achieved only by putting its surface in contact with a completely CO2-free environment. On the contrary, similarly modified MOFs show higher CO2 adsorption working capacities: this potentially makes them even better candidates than their mesoporous inorganic homologues for a plant scale use. However, the persisting lack of reliable methods for the pelletization of both ordered mesoporous silicates and MOFs creates a care for further development efforts in the next future.

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Authors: Gargiulo, N., Pepe, F., & Caputo, D.
ORCID: Gargiulo, Nicola
Pepe, Francesco
Caputo, Domenico
Venue: Journal of Nanoscience and Nanotechnology
Publisher: American Scientific Publishers
Published: 2014-02-01
Volume: 14
Issue: 2
Pages: 1811-1822
ISSN: 1533-4880 (ISSN-L)
1533-4899
DOI: 10.1166/jnn.2014.8893
OpenAlex: W2326306759
Cited by: 117
References: 0
Citations by year: 2026: 3 · 2025: 6 · 2024: 12 · 2023: 8 · 2022: 10 · 2021: 10 · 2020: 13 · 2019: 12 · 2018: 10 · 2017: 7 · 2016: 10 · 2015: 10 · 2014: 6
FWCI: 12.79
Type: journal article
Language: en
Open access: closed
Locations: Journal of Nanoscience and Nanotechnology (publishedVersion)
PubMed (publishedVersion)
Topics: Physical Sciences › Chemical Engineering › Filtration and Separation › Carbon Dioxide Capture Technologies
Physical Sciences › Chemistry › Inorganic Chemistry › Metal-Organic Frameworks: Synthesis and Applications
Physical Sciences › Chemistry › Inorganic Chemistry › Zeolite Catalysis and Synthesis
Keywords: CO2 adsorption, CO2 capture, zeolites, cation-exchanged zeolites, mesoporous silicates, metal-organic frameworks, amino-functionalized MOF, adsorbent regeneration, pelletization
MeSH terms: Adsorption, Carbon Dioxide, Materials Testing, Molecular Conformation, Particle Size, Surface Properties, Nanostructures, Nanopores

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CO2 Adsorption by Functionalized Nanoporous Materials: A Review

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