The DOI matches its Crossref record; 32 of the 32 references it cites were found in a registry or an index.
Plasmon-exciton-polariton lasing
Open accessAbstract
Metallic nanostructures provide a toolkit for the generation of coherent light below the diffraction limit. Plasmonic based lasing relies on the population inversion of emitters (such as organic fluorophores) along with feedback provided by plasmonic resonances. In this regime, known as weak light matter coupling, the radiative characteristics of the system can be described by the Purcell effect. Strong light matter coupling between the molecular excitons and electromagnetic field generated by the plasmonic structures leads to the formation of hybrid quasi-particles known as plasmon exciton polaritons (PEPs). Due to the bosonic character of these quasi particles, exciton polariton condensation can lead to laser-like emission at much lower threshold powers than in conventional photon lasers. Here, we observe PEP lasing through a dark plasmonic mode in an array of metallic nanoparticles with a low threshold in an optically pumped organic system. Interestingly, the threshold power of the lasing is reduced by increasing the degree of light matter coupling in spite of the degradation of the quantum efficiency of the active material, highlighting the ultrafast dynamic responsible for the lasing, i.e., stimulated scattering. These results demonstrate a unique roomtemperature platform for exploring the physics of exciton polaritons in an open cavity architecture and pave the road toward the integration of this on-chip lasing device with the current photonics and active metamaterial planar technologies.
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Citations
Cites
Bose–Einstein condensation of exciton polaritons
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Colloquium: Light scattering by particle and hole arrays
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Superfluidity of polaritons in semiconductor microcavities
Amo, A., Lefrère, J., Pigeon, S., Adrados, C., Ciuti, C., Carusotto, I., Houdré, R., Giacobino, E., & Bramati, A. (2009) · Nature Physics · doi:10.1038/nphys1364 · Cited by 1,037
Room-Temperature Polariton Lasing in Semiconductor Microcavities
Christopoulos, S., von Högersthal, G. B. H., Grundy, A. J. D., Lagoudakis, P. G., Kavokin, A. V., Baumberg, J. J., Christmann, G., Butté, R., Feltin, E., Carlin, J.-F., et al. (2007) · Physical Review Letters · doi:10.1103/physrevlett.98.126405 · Cited by 1,020
Room-Temperature Polariton Lasing in an Organic Single-Crystal Microcavity
Kéna-Cohen, S., & Forrest, S. R. (2010) · Nature Photonics · doi:10.1038/nphoton.2010.86 · Cited by 942 · cited 2×
“This implies that organic exciton-polariton lasing is most efficient when the relaxation from the reservoir to the lasing state is resonant with a strong optical phonon line [14].”
BackgroundStrong exciton–photon coupling in an organic semiconductor microcavity
Lidzey, D. G., Bradley, D. D. C., Skolnick, M. S., Virgili, T., Walker, S., & Whittaker, D. M. (1998) · Nature · doi:10.1038/25692 · Cited by 926
Strong Coupling between Surface Plasmons and Excitons in an Organic Semiconductor
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Lasing action in strongly coupled plasmonic nanocavity arrays
Zhou, W., Dridi, M., Suh, J. Y., Kim, C. H., Co, D. T., Wasielewski, M. R., Schatz, G. C., & Odom, T. W. (2013) · Nature Nanotechnology · doi:10.1038/nnano.2013.99 · Cited by 803
Cited by
Non-equilibrium Bose–Einstein condensation in photonic systems
Bloch, J., Carusotto, I., & Wouters, M. (2022) · Nature Reviews Physics · doi:10.1038/s42254-022-00464-0 · Cited by 105
Unstable and stable regimes of polariton condensation
Baboux, F., De Bernardis, D., Goblot, V., Gladilin, V. N., Gomez, C., Galopin, E., Le Gratiet, L., Lemaître, A., Sagnes, I., Carusotto, I., et al. (2018) · Optica · doi:10.1364/optica.5.001163 · Cited by 79
Metadata
- Authors
- Ramezani, M., Halpin, A., Fernández-Domínguez, A. I., Feist, J., Rodriguez, S. R.-K., Garcia-Vidal, F. J., & Gómez Rivas, J.
- Venue
- Optica
- Publisher
- Optica Publishing Group
- Published
- 2016-12-22
- Volume
- 4
- Issue
- 1
- Pages
- 31
- ISSN
- 2334-2536 (ISSN-L)
- OpenAlex
- W2465098511
- Cited by
- 258
- References
- 32
- FWCI
- 13.34
- Type
- journal article
- Language
- en
- Open access
- gold
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- Ramezani, M., Halpin, A., Fernández-Domínguez, A. I., Feist, J., Rodriguez, S. R.-K., Garcia-Vidal, F. J., & Gómez Rivas, J. (2017). Plasmon-exciton-polariton lasing. Optica. https://doi.org/10.1364/optica.4.000031
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