Cited by 333Atmospheric chemistry and aerosolsAtmospheric Ozone and ClimateAtmospheric and Environmental Gas Dynamics

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Significant increase of surface ozone at a rural site, north of eastern China

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Ma, Zhiqiang, Xu, Jing, Quan, Weijun, Zhang, Ziyin, Lin, Weili, Xu, Xiaobin·2016·Atmospheric chemistry and physics

DOI 10.5194/acp-16-3969-2016

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Abstract

Abstract. Ozone pollution has become one of the top environmental concerns in eastern China. Quantifying temporal trend of surface ozone concentrations is very meaningful to assess the impacts of the anthropogenic precursor reductions and the effects of emission control strategies. The level of surface ozone is impacted by both emissions of precursors and meteorological conditions. In order to examine the variation trend of ozone from 2003 to 2015 in Shangdianzi regional atmosphere background station, the modified KZ filter method was performed in this study to remove the influence of meteorological fluctuations on ozone concentrations. Results reveal that the short-term component, seasonal component and long-term component of ozone account for 36.4, 57.6 and 2.2 % of the total variance, respectively. The long-term trend shows that the surface daily maximum 8-h O3 has undergone a significant increase during 2003–2015, with a rate of 1.1 ppb yr−1. We find that the increase was completely resulted from the change of the emissions when the influence of the meteorological factors was eliminated. Furthermore, the variation of NO2 indicated that VOCs seemed to play more important role in the increase trend of the surface ozone.

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Figure 2 Separated time series of MDA8 values of ozone at SDZ: (a) the original data; (b) the short-term component, W.t/ ; (c) the seasonal component, S.t/ ; (d) the long-term component, e.t/ .CC-BY · From the PDF

Figure 3 Q -Q plot of the short-term component W.t/ for ozone.CC-BY · From the PDF

Figure 4 Separated time series of daily mean values of temperature at SDZ: (a) the original data; (b) the short-term component, W.t/ ; (c) the seasonal component, S.t/ ; (d) the long-term component, e.t/ .CC-BY · From the PDF

Figure 5 Results of the daily mean temperature and the MDA8 value of ozone after the application of the KZ 15 ; 5 filter to the original time series. The results indicate the sum of the seasonal and long-term components.CC-BY · From the PDF

Figure 6 Linear regression fit on the filtered daily maxima of temperature and ozone. Temperature data are lagged by 17 days to ozone data.CC-BY · From the PDF

Figure 7 Time series of the noise-free and temperatureindependent ozone. The red line is a linear fit and the blue lines are the 95 % confidence prediction band.CC-BY · From the PDF

Figure 8 Long-term trends of NO 2 and the MDA8 ozone value calculated by KZ 365 ; 3 :CC-BY · From the PDF

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Authors: Ma, Z., Xu, J., Quan, W., Zhang, Z., Lin, W., & Xu, X.
Affiliations: China Meteorological Administration (CN)
Chinese Academy of Meteorological Sciences (CN)
Corresponding author: Lin, Weili
ORCID: Ma, Zhiqiang
Xu, Jing
Quan, Weijun
Zhang, Ziyin
Lin, Weili
Xu, Xiaobin
Venue: Atmospheric chemistry and physics
Publisher: Copernicus GmbH
Published: 2016-03-24
Volume: 16
Issue: 6
Pages: 3969-3977
ISSN: 1680-7316 (ISSN-L)
1680-7324
DOI: 10.5194/acp-16-3969-2016
OpenAlex: W2304410378
Cited by: 332
References: 52
Citations by year: 2026: 6 · 2025: 21 · 2024: 30 · 2023: 42 · 2022: 52 · 2021: 50 · 2020: 49 · 2019: 40 · 2018: 21 · 2017: 16 · 2016: 5
FWCI: 16.68
Type: journal article
Language: en
Open access: gold
doi.org
Licence: cc-by
creativecommons.org/licenses/by/3.0/ (vor)
Locations: Atmospheric chemistry and physics (publishedVersion, cc-by)
DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
Funders: National Natural Science Foundation of China (41475135)
Natural Science Foundation of Beijing Municipality (8132025, 8152018)
Topics: Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › Atmospheric chemistry and aerosols
Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › Atmospheric Ozone and Climate
Physical Sciences › Environmental Science › Global and Planetary Change › Atmospheric and Environmental Gas Dynamics
Keywords: surface ozone, ozone trends, North China Plain, VOC emissions, NO2, seasonal ozone variation

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Significant increase of surface ozone at a rural site, north of eastern China

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