Pan-Arctic aerosol number size distributions: seasonality and transport patterns
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Abstract
Abstract. The Arctic environment has an amplified response to global climatic change. It is sensitive to human activities that mostly take place elsewhere. For this study, a multi-year set of observed aerosol number size distributions in the diameter range of 10 to 500 nm from five sites around the Arctic Ocean (Alert, Villum Research Station – Station Nord, Zeppelin, Tiksi and Barrow) was assembled and analysed.A cluster analysis of the aerosol number size distributions revealed four distinct distributions. Together with Lagrangian air parcel back-trajectories, they were used to link the observed aerosol number size distributions with a variety of transport regimes. This analysis yields insight into aerosol dynamics, transport and removal processes, on both an intra- and an inter-monthly scale. For instance, the relative occurrence of aerosol number size distributions that indicate new particle formation (NPF) event is near zero during the dark months, increases gradually to ∼ 40 % from spring to summer, and then collapses in autumn. Also, the likelihood of Arctic haze aerosols is minimal in summer and peaks in April at all sites.The residence time of accumulation-mode particles in the Arctic troposphere is typically long enough to allow tracking them back to their source regions. Air flow that passes at low altitude over central Siberia and western Russia is associated with relatively high concentrations of accumulation-mode particles (Nacc) at all five sites – often above 150 cm−3. There are also indications of air descending into the Arctic boundary layer after transport from lower latitudes.The analysis of the back-trajectories together with the meteorological fields along them indicates that the main driver of the Arctic annual cycle of Nacc, on the larger scale, is when atmospheric transport covers the source regions for these particles in the 10-day period preceding the observations in the Arctic. The scavenging of these particles by precipitation is shown to be important on a regional scale and it is most active in summer. Cloud processing is an additional factor that enhances the Nacc annual cycle.There are some consistent differences between the sites that are beyond the year-to-year variability. They are the result of differences in the proximity to the aerosol source regions and to the Arctic Ocean sea-ice edge, as well as in the exposure to free-tropospheric air and in precipitation patterns – to mention a few. Hence, for most purposes, aerosol observations from a single Arctic site cannot represent the entire Arctic region. Therefore, the results presented here are a powerful observational benchmark for evaluation of detailed climate and air chemistry modelling studies of aerosols throughout the vast Arctic region.
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Freud et al. (2017) reported concentrations 190-250 cm-3 in size range 10-500 nm at Utqiaġvik/Barrow for Jan-Feb.
“Additionally, Freud et al. (2017) reported concentrations between roughly 190 and 250 cm -3 in the size range 10 to 500 nm at Utqiaġvik/Barrow for the months of January and February.”
From In situ vertical observations of the layered structure of air pollution in a continental high-latitude urban boundary layer during winter (2025) · cites this paper as Freud et al. (2017)
Section 3.1 describes monthly total aerosol number concentrations for particles from 10 to 500 nm, and section 3.2 discusses monthly distributions at Barrow. The passages in our copy do not state the claimed January–February concentrations of roughly 190–250 cm⁻³; searches for those values and months did not establish them. (LLM, conf=0.78)
Experimental — accuracy not yet measuredThe observed LBL distribution is very similar to the distribution observed by Freud et al. (2017) at Utqiaġvik/Barrow for January and February and to their accumulation mode cluster representative of Arctic haze.
“The observed distribution is very similar to the distribution observed by Freud et al. (2017) at Utqiaġvik/Barrow for the months of January and February and to their accumulation mode cluster (cluster 1) representative of Arctic haze.”
From In situ vertical observations of the layered structure of air pollution in a continental high-latitude urban boundary layer during winter (2025) · cites this paper as Freud et al. (2017)
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Self-citationAerosol and dynamical contributions to cloud droplet formation in Arctic low-level clouds
Motos, G., Freitas, G. P., Georgakaki, P., Wieder, J., Li, G., Aas, W., Lunder, C., Krejčí, R., Pasquier, J. T., Henneberger, J., et al. (2023) · Atmospheric chemistry and physics · doi:10.5194/acp-23-13941-2023 · Cited by 15 · see citing works
Gilardoni, S., Heslin‐Rees, D., Mazzola, M., Vitale, V., Sprenger, M. A., & Krejčí, R. (2023) · Atmospheric chemistry and physics · doi:10.5194/acp-23-15589-2023 · Cited by 15 · see citing works
Ahn, S. H., Yoon, Y. J., Choi, T., Lee, J. Y., Kim, Y. P., Lee, B. Y., Ritter, C., Aas, W., Krejčí, R., Ström, J., et al. (2021) · Atmospheric Environment · doi:10.1016/j.atmosenv.2021.118748 · Cited by 14 · see citing works
Self-citationHeutte, B., Bergner, N., Angot, H., Pernov, J., Dada, L., Mirrielees, J. A., Beck, I., Baccarini, A., Boyer, M., Creamean, J. M., et al. (2025) · Atmospheric chemistry and physics · doi:10.5194/acp-25-2207-2025 · Cited by 14 · see citing works
Potential Source Areas for Atmospheric Lead Reaching Ny-Ålesund from 2010 to 2018
Bazzano, A., Bertinetti, S., Ardini, F., Cappelletti, D., & Grotti, M. (2021) · Atmosphere · doi:10.3390/atmos12030388 · Cited by 14 · see citing works
Pohorsky, R., Baccarini, A., Brett, N., Barret, B., Bekki, S., Pappaccogli, G., Dieudonné, E., Temime-Roussel, B., D'Anna, B., Cesler-Maloney, M., et al. (2025) · Atmospheric Chemistry and Physics · doi:10.5194/acp-25-3687-2025 · Cited by 12 · see citing works
Indirect Measurements of the Composition of Ultrafine Particles in the Arctic Late‐Winter
Myers, D. C., Lawler, M. J., Mauldin, R. L., Sjostedt, S. J., Dubey, M. K., Abbatt, J. P. D., & SMITH, J. N. M. (2021) · Journal of Geophysical Research Atmospheres · doi:10.1029/2021jd035428 · Cited by 12 · see citing works
Hansson, H., Tunved, P., Krejčí, R., Freud, E., Kalivitis, N., Hennig, T., Maneas, G., & Gerasopoulos, E. (2021) · Atmosphere · doi:10.3390/atmos12040445 · Cited by 12 · see citing works
Self-citationEngsvang, M., Wu, H., & Elm, J. (2024) · ACS Omega · doi:10.1021/acsomega.4c01235 · Cited by 11 · see citing works
Adachi, K., Tobo, Y., Oshima, N., Yoshida, A., Ohata, S., Krejčí, R., Maßling, A., Skov, H., & Koike, M. (2023) · Atmospheric Environment · doi:10.1016/j.atmosenv.2023.120083 · Cited by 11 · see citing works
Self-citationObserved aerosol‐layer depth at Station Nord in the high Arctic
Gryning, S., Batchvarova, E., Floors, R., Münkel, C., Sørensen, L. L., & Skov, H. (2023) · International Journal of Climatology · doi:10.1002/joc.8027 · Cited by 11 · see citing works
Self-citationHeslin‐Rees, D., Tunved, P., Ström, J., Cremer, R. S., Zieger, P., Riipinen, I., Ekman, A. M. L., Eleftheriadis, K., & Krejčí, R. (2024) · Atmospheric chemistry and physics · doi:10.5194/acp-24-2059-2024 · Cited by 10 · see citing works
Self-citationPan-Arctic methanesulfonic acid aerosol: source regions, atmospheric drivers, and future projections
Pernov, J., Harris, E., Volpi, M., Baumgartner, T., Hohermuth, B., Henne, S., Aeberhard, W. H., Becagli, S., Quinn, P. K., Traversi, R., et al. (2024) · npj Climate and Atmospheric Science · doi:10.1038/s41612-024-00712-3 · Cited by 10 · see citing works
Boyer, M., Aliaga, D., Quéléver, L. L. J., Bucci, S., Angot, H., Dada, L., Heutte, B., Beck, L., Dütsch, M., Stohl, A., et al. (2024) · Atmospheric chemistry and physics · doi:10.5194/acp-24-12595-2024 · Cited by 10 · see citing works
Vicente-Luis, A., Tremblay, S., Dionne, J., Chang, R., Fogal, P. F., Leaitch, W. R., Sharma, S., Kolonjari, F., & Hayes, P. L. (2021) · Atmospheric Environment · doi:10.1016/j.atmosenv.2021.118254 · Cited by 10 · see citing works
Processes contributing to cloud dissipation and formation events on the North Slope of Alaska
Sedlar, J., Igel, A. L., & Telg, H. (2021) · Atmospheric chemistry and physics · doi:10.5194/acp-21-4149-2021 · Cited by 10 · see citing works
Dekhtyareva, A., Hermanson, M. H., Nikulina, A., Hermansen, O., Svendby, T., Holmén, K. J., & Graversen, R. G. (2022) · Atmospheric chemistry and physics · doi:10.5194/acp-22-11631-2022 · Cited by 10 · see citing works
Canadian high arctic ice core records of organophosphate flame retardants and plasticizers
Silva, A. O. D., Young, C. J., Spencer, C., Muir, D. C. G., Sharp, M. J., Lehnherr, I., & Criscitiello, A. S. (2023) · Environmental Science Processes & Impacts · doi:10.1039/d3em00215b · Cited by 9 · see citing works
Spolaor, A., Barbaro, E., Mazzola, M., Viola, A. P., Lisok, J., Obleitner, F., Markowicz, K. M., & Cappelletti, D. (2017) · Atmospheric Environment · doi:10.1016/j.atmosenv.2017.09.042 · Cited by 9 · see citing works
Doulgeris, K., Vakkari, V., O'Connor, E. J., Kerminen, V., Lihavainen, H., & Brus, D. (2023) · Atmospheric chemistry and physics · doi:10.5194/acp-23-2483-2023 · Cited by 7 · see citing works
Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic
Williams, A. S., Dedrick, J. L., Russell, L. M., Tornow, F., Silber, I., Fridlind, A. M., Swanson, B., DeMott, P. J., Zieger, P., & Krejčí, R. (2024) · Atmospheric chemistry and physics · doi:10.5194/acp-24-11791-2024 · Cited by 7 · see citing works
Impacts of sea ice leads on sea salt aerosols and atmospheric chemistry in the Arctic
Emme, E. J., & Horowitz, H. M. (2025) · Atmospheric chemistry and physics · doi:10.5194/acp-25-4531-2025 · Cited by 6 · see citing works
Engsvang, M., & Elm, J. (2025) · ACS Omega · doi:10.1021/acsomega.5c02147 · Cited by 6 · see citing works
Aerosol processes in high-latitude environments and the effects on climate
Ekman, A. M. L., & Schmale, J. (2022) · Elsevier eBooks · doi:10.1016/b978-0-12-819766-0.00005-5 · Cited by 6 · see citing works
Seasonal dynamics of airborne biomolecules influence the size distribution of Arctic aerosols
Jang, E., Park, K., Yoon, Y. J., Jang, K., Kim, M. S., Kim, K., Chung, H. Y., Mazzola, M., Cappelletti, D., & Lee, B. Y. (2024) · Environmental Science and Ecotechnology · doi:10.1016/j.ese.2024.100458 · Cited by 5 · see citing works
Aerosol hygroscopicity influenced by seasonal chemical composition variations in the Arctic region
Kang, H., Jung, C. H., Lee, B., Krejčí, R., Heslin‐Rees, D., Aas, W., & Yoon, Y. J. (2025) · Journal of Aerosol Science · doi:10.1016/j.jaerosci.2025.106551 · Cited by 5 · see citing works
Lee, J. Y., Xian, P., Selimovic, V., Booth, P.-P. M., Anderson, B. G., Liu, J., & Pratt, K. A. (2025) · ACS Earth and Space Chemistry · doi:10.1021/acsearthspacechem.5c00172 · Cited by 4 · see citing works
Hasager, F., Nielsen, O. J., & Mikkelsen, K. V. (2022) · Environmental Science Atmospheres · doi:10.1039/d1ea00105a · Cited by 4 · see citing works
Guy, H., Martin, A. S., Olson, E., Brooks, I. M., & Neely, R. R. (2024) · Atmospheric chemistry and physics · doi:10.5194/acp-24-11103-2024 · Cited by 3 · see citing works
Size-separated aerosol chemical characterization over Ny-Ålesund during the Arctic summer of 2010
Sonbawne, S. M., Raju, M. P., Safai, P. D., Devara, P. C. S., Fadnavis, S. S., Panicker, A. S., & Pandithurai, G. (2023) · Sustainable Chemistry for Climate Action · doi:10.1016/j.scca.2023.100016 · Cited by 3 · see citing works
Dynamics of gaseous oxidized mercury at Villum Research Station during the High Arctic summer
Pernov, J., Jensen, B., Maßling, A., Thomas, D. C., & Skov, H. (2021) · Atmospheric chemistry and physics · doi:10.5194/acp-21-13287-2021 · Cited by 3 · see citing works
Self-citationSources and Composition of Organic Aerosols in the Central Arctic during Spring and Summer
Heutte, B., Angot, H., Chen, G., Pernov, J., Haddad, I. E., Dada, L., Daellenbach, K. R., Beck, I., Bergner, N., Bucci, S., et al. (2025) · Environmental Science & Technology · doi:10.1021/acs.est.5c09788 · Cited by 2 · see citing works
- Authors
- Freud, E., Krejci, R., Tunved, P., Leaitch, R., Nguyen, Q. T., Massling, A., Skov, H., & Barrie, L.
- Affiliations
- Stockholm University (SE)
- Aarhus University (DK)
- Corresponding author
- Freud, Eyal
- ORCID
- Venue
- Atmospheric Chemistry and Physics
- Publisher
- Copernicus GmbH
- Published
- 2017-07-04
- Volume
- 17
- Issue
- 13
- Pages
- 8101-8128
- ISSN
- 1680-7316 (ISSN-L)
- 1680-7324
- OpenAlex
- W2586516499
- Cited by
- 169
- References
- 90
- Citations by year
- 2026: 8 · 2025: 16 · 2024: 11 · 2023: 21 · 2022: 35 · 2021: 40 · 2020: 10 · 2019: 13 · 2018: 11 · 2017: 4
- FWCI
- 6.82
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- Locations
- Atmospheric chemistry and physics (publishedVersion, cc-by)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Funders
- Villum Fonden
- Svenska Forskningsrådet Formas
- Naturvårdsverket
- Vetenskapsrådet
- Miljøstyrelsen
- Ministère de la Défense Nationale
- National Oceanic and Atmospheric Administration
- Topics
- Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › Atmospheric chemistry and aerosols
- Physical Sciences › Environmental Science › Global and Planetary Change › Atmospheric aerosols and clouds
- Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › Atmospheric Ozone and Climate
- Keywords
- Arctic aerosols, aerosol number size distribution, new particle formation, Arctic haze, accumulation mode particles, aerosol transport, Lagrangian back trajectories, seasonal cycle, precipitation scavenging, cloud processing, Arctic boundary layer, sea ice edge, Arctic climate change
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