Porous Platinum Nanotubes for Oxygen Reduction and Methanol Oxidation Reactions
Abstract
Porous platinum nanotubes (PtNTs) with a all thickness of 5 nm, an outer diameter of 60 nm, and a length of 5–20 μm are synthesized by galvanic displacement with silver nanowires, which are formed by the ethylene glycol reduction of silver nitrate. Oxygen reduction reaction (ORR) and durability experiments are conducted for PtNTs, Pt nanoparticles supported on carbon (Pt/C), and bulk polycrystalline Pt (BP‐Pt) electrocatalysts to evaluate their catalytic properties for use as cathode catalysts in proton exchange membrane fuel cells. PtNTs demonstrate improved mass and specific activity for ORR and durability to Pt/C. Following durability testing, PtNTs exhibit specific ORR activity approaching that of BP‐Pt. Catalyst activity for the methanol oxidation reaction (MOR) is characterized through cyclic voltammetry and chronoamperometry techniques to evaluate the materials for use as anode catalysts in direct methanol fuel cells. The PtNTs show improved specific activity for MOR and chronoamperometry characteristics over Pt/C and BP‐Pt catalysts.
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Carbon support material corrosion can degrade catalyst, causing catalyst NPs to detach from the support and sinter on the membrane, leading to poor fuel cell performance.
“the carbon support materials corrosive specification can degrade catalyst, as a resulting catalyst NPs detach from the support and sinter on the membrane, leading to poor fuel cell performance.”
From Renewable energy harvesting with the application of nanotechnology: A review (2019) · cites this paper as [119]
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- Authors
- Alia, S. M., Zhang, G., Kisailus, D., Li, D., Gu, S., Jensen, K., & Yan, Y.
- Affiliations
- University of California, Riverside (US)
- Jilin University (CN)
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2010-10
- Volume
- 20
- Issue
- 21
- Pages
- 3742-3746
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2056657180
- Cited by
- 269
- References
- 32
- Citations by year
- 2026: 6 · 2025: 8 · 2024: 3 · 2023: 5 · 2022: 9 · 2021: 12 · 2020: 15 · 2019: 16 · 2018: 21 · 2017: 20 · 2016: 28 · 2015: 27 · 2014: 29 · 2013: 31 · 2012: 25
- FWCI
- 10.46
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Advanced Functional Materials (publishedVersion)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Keywords
- oxygen reduction reaction, methanol oxidation, galvanic replacement, silver nanowires, ethylene glycol reduction, platinum electrocatalysts, proton exchange membrane fuel cells, direct methanol fuel cells, catalyst stability, mass and specific activity, Pt/C comparison
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