An Interface‐Induced Co‐Assembly Approach Towards Ordered Mesoporous Carbon/Graphene Aerogel for High‐Performance Supercapacitors

Liu, Ruili; Wan, Li; Liu, Shaoqing; Pan, Lixia; Wu, Dongqing; Zhao, Dongyuan

doi:10.1002/adfm.201403280

Cited by 238Supercapacitor Materials and FabricationMesoporous Materials and CatalysisAerogels and thermal insulation

An Interface‐Induced Co‐Assembly Approach Towards Ordered Mesoporous Carbon/Graphene Aerogel for High‐Performance Supercapacitors

Liu, Ruili, Wan, Li, Liu, Shaoqing, Pan, Lixia, Wu, Dongqing, Zhao, Dongyuan·2015·Advanced Functional Materials

DOI 10.1002/adfm.201403280

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Abstract

Hierarchically porous composites with mesoporous carbon wrapping around the macroporous graphene aerogel can combine the advantages of both components and are expected to show excellent performance in electrochemical energy devices. However, the fabrication of such composites is challenging due to the lack of an effective strategy to control the porosity of the mesostructured carbon layers. Here an interface‐induced co‐assembly approach towards hierarchically mesoporous carbon/graphene aerogel composites, possessing interconnected macroporous graphene networks covered by highly ordered mesoporous carbon with a diameter of ≈9.6 nm, is reported. And the orientation of the mesopores (vertical or horizontal to the surface of the composites) can be tuned by the ratio of the components. As the electrodes in supercapacitors, the resulting composites demonstrate outstanding electrochemical performances. More importantly, the synthesis strategy provides an ideal platform for hierarchically porous graphene composites with potential for energy storage and conversion applications.

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Carbon aerogel (CA) with a 3D interconnected network and unique properties, including highly porous structure, large surface area, and great electron transport performance, is an ideal substrate for MoS2 loading and can be used in the energy area.
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From In-Situ Growth of Few-Layered MoS2 Nanosheets on Highly Porous Carbon Aerogel as Advanced Electrocatalysts for Hydrogen Evolution Reaction (2015) · cites this paper as [44]

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Supercapacitors: An Interface‐Induced Co‐Assembly Approach Towards Ordered Mesoporous Carbon/Graphene Aerogel for High‐Performance Supercapacitors (Adv. Funct. Mater. 4/2015)
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Authors: Liu, R., Wan, L., Liu, S., Pan, L., Wu, D., & Zhao, D.
Affiliations: Shanghai University (CN)
Shanghai Jiao Tong University (CN)
Fudan University (CN)
Corresponding author: Liu, Ruili
Wu, Dongqing
ORCID: Liu, Ruili
Wan, Li
Liu, Shaoqing
Wu, Dongqing
Zhao, Dongyuan
Venue: Advanced Functional Materials
Publisher: Wiley
Published: 2014-11-19
Volume: 25
Issue: 4
Pages: 526-533
ISSN: 1616-301X (ISSN-L)
1616-3028
DOI: 10.1002/adfm.201403280
OpenAlex: W2033989787
Cited by: 238
References: 51
Citations by year: 2026: 5 · 2025: 4 · 2024: 7 · 2023: 14 · 2022: 11 · 2021: 27 · 2020: 23 · 2019: 34 · 2018: 32 · 2017: 30 · 2016: 37 · 2015: 14
FWCI: 9.13
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Advanced Functional Materials (publishedVersion)
Topics: Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
Physical Sciences › Materials Science › Materials Chemistry › Mesoporous Materials and Catalysis
Physical Sciences › Chemistry › Spectroscopy › Aerogels and thermal insulation
Keywords: mesoporous carbon, graphene aerogel, hierarchical porous composites, supercapacitor electrodes, energy storage

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An Interface‐Induced Co‐Assembly Approach Towards Ordered Mesoporous Carbon/Graphene Aerogel for High‐Performance Supercapacitors

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