The DOI matches its Crossref record; 58 of the 58 references it cites were found in a registry or an index.
Semisacrificial Template Growth of Self‐Supporting MOF Nanocomposite Electrode for Efficient Electrocatalytic Water Oxidation
Abstract
Herein, the authors report, for the first time, the semisacrificial template growth of a self‐supporting metal–organic framework (MOF) nanocomposite electrode composed of ultrasmall iron‐rich Fe(Ni)‐MOF cluster‐decorated ultrathin Ni‐rich Ni(Fe)‐MOF nanosheets from the NiFe alloy foam, in which the Fe(Ni)‐MOF clusters are uniform with a particle size of 2–5 nm, while the thickness of the Ni(Fe)‐MOF nanosheets is only about 1.56 nm. When directly used as a self‐supported working electrode for the oxygen evolution reaction (OER), it can afford an impressive electrocatalytic performance with required overpotentials of 227 and 253 mV to achieve current densities of 10 and 100 mA cm−2, respectively, much outperforming the benchmark of RuO 2 and most state‐of‐the‐art noble‐metal‐free catalysts. Characterizations demonstrated that the combination of the unique nanostructure of the catalyst and the strong coupling effect between Ni and Fe active sites should be responsible for its excellent OER performance. Remarkably, when coupled with a Pt electrode in an overall water splitting system, they only needed 1.537 V to achieve a current density of 10 mA cm−2. The facile and economical methodology represents a new way to design and prepare high‐performance self‐supporting MOF electrocatalysts for highly efficient electrochemical processes.
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Cites
Ultrathin metal–organic framework nanosheets for electrocatalytic oxygen evolution
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Metal-organic framework nanosheets as building blocks for molecular sieving membranes
Peng, Y., Li, Y., Ban, Y., Jin, H., Jiao, W., Liu, X., & Yang, W. (2014) · Science · doi:10.1126/science.1254227 · Cited by 1,731
Ni2P as a Janus catalyst for water splitting: the oxygen evolution activity of Ni2P nanoparticles
Stern, L.-A., Feng, L., Song, F., & Hu, X. (2015) · Energy & Environmental Science · doi:10.1039/c5ee01155h · Cited by 1,616
Emerging Multifunctional Metal–Organic Framework Materials
Li, B., Wen, H., Cui, Y., Zhou, W., Qian, G., & Chen, B. (2016) · Advanced Materials · doi:10.1002/adma.201601133 · Cited by 1,587
Ultrathin metal-organic framework array for efficient electrocatalytic water splitting
Duan, J., Chen, S., & Zhao, C. (2017) · Nature Communications · doi:10.1038/ncomms15341 · Cited by 1,319
Nanomaterials derived from metal–organic frameworks
Dang, S., Zhu, Q.-L., & Xu, Q. (2017) · Nature Reviews Materials · doi:10.1038/natrevmats.2017.75 · Cited by 1,230
Self-citationMetal-Organic Frameworks for Energy Applications
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Self-citationUltrathin 2D Metal–Organic Framework Nanosheets
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Metal–Organic Frameworks for Electrocatalytic Reduction of Carbon Dioxide
Kornienko, N., Zhao, Y., Kley, C. S., Zhu, C., Kim, D., Lin, S., Chang, C. J., Yaghi, O. M., & Yang, P. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08212 · Cited by 1,158
Cited by
Metal–organic frameworks and their derivatives as electrocatalysts for the oxygen evolution reaction
Du, J., Li, F., & Sun, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01191f · Cited by 578
Cao, C., Ma, D., Gu, J., Xie, X., Zeng, G., Li, X., Han, S., Zhu, Q., Wu, X., & Xu, Q. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202005577 · Cited by 417
Self-citationKarimi-Maleh, H., Yola, M. L., Atar, N., Orooji, Y., Karimi, F., Senthil Kumar, P., Rouhi, J., & Baghayeri, M. (2021) · Journal of Colloid and Interface Science · doi:10.1016/j.jcis.2021.02.066 · Cited by 404
Electrochemical synergies of Fe–Ni bimetallic MOF CNTs catalyst for OER in water splitting
Yaqoob, L., Noor, T., Iqbal, N., Nasir, H., Zaman, N., & Talha, K. (2021) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2020.156583 · Cited by 258
Metadata
- Authors
- Cao, C., Ma, D., Xu, Q., Wu, X., & Zhu, Q.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2018-12-13
- Volume
- 29
- Issue
- 6
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2903615107
- Cited by
- 313
- References
- 58
- FWCI
- 8.65
- Type
- journal article
- Language
- en
- Open access
- closed
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- Cao, C., Ma, D., Xu, Q., Wu, X., & Zhu, Q. (2019). Semisacrificial Template Growth of Self‐Supporting MOF Nanocomposite Electrode for Efficient Electrocatalytic Water Oxidation. Advanced Functional Materials. https://doi.org/10.1002/adfm.201807418
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