The DOI matches its Crossref record; 62 of the 62 references it cites were found in a registry or an index.
Metal–Organic Layers Leading to Atomically Thin Bismuthene for Efficient Carbon Dioxide Electroreduction to Liquid Fuel
Abstract
Electrochemical reduction of CO 2 to valuable fuels is appealing for CO 2 fixation and energy storage. However, the development of electrocatalysts with high activity and selectivity in a wide potential window is challenging. Herein, atomically thin bismuthene (Bi‐ene) is pioneeringly obtained by an in situ electrochemical transformation from ultrathin bismuth‐based metal–organic layers. The few‐layer Bi‐ene, which possesses a great mass of exposed active sites with high intrinsic activity, has a high selectivity (ca. 100 %), large partial current density, and quite good stability in a potential window exceeding 0.35 V toward formate production. It even deliver current densities that exceed 300.0 mA cm−2 without compromising selectivity in a flow‐cell reactor. Using in situ ATR‐IR spectra and DFT analysis, a reaction mechanism involving HCO 3− for formate generation was unveiled, which brings new fundamental understanding of CO 2 reduction.
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1 retracted
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Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
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Self-citationWu, Z., Wu, H., Cai, W., Wen, Z., Jia, B., Wang, L., Jin, W., & Ma, T. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202102832 · Cited by 354
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Yao, D., Tang, C., Vasileff, A., Zhi, X., Jiao, Y., & Qiao, S. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202104747 · Cited by 312
Metadata
- Authors
- Cao, C., Ma, D., Gu, J., Xie, X., Zeng, G., Li, X., Han, S., Zhu, Q., Wu, X., & Xu, Q.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-06-10
- Volume
- 59
- Issue
- 35
- Pages
- 15014-15020
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4246047186
- Cited by
- 417
- References
- 62
- FWCI
- 12.53
- Type
- journal article
- Language
- en
- Open access
- closed
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- Cao, C., Ma, D., Gu, J., Xie, X., Zeng, G., Li, X., Han, S., Zhu, Q., Wu, X., & Xu, Q. (2020). Metal–Organic Layers Leading to Atomically Thin Bismuthene for Efficient Carbon Dioxide Electroreduction to Liquid Fuel. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202005577
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