The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Electrolytes Enriched by Crown Ethers for Lithium Metal Batteries
Abstract
Lithium (Li) metal battery is considered the most promising next‐generation battery due to its low potential and high theoretical capacity. However, Li dendrite growth causes serious safety problems. Herein, the 15‐Crown‐5 (15‐C‐5) is reported as an electrolyte additive based on solvation shell regulation. The strong complex effect between Li+ ion and 15‐C‐5 can reduce the concentration of Li ions on the electrode surface, thus changing the nucleation, and repressing the growth of Li dendrites in the plating process. Significantly, the strong coordination of Li+/15‐C‐5 would be able to make them aggregate around the Li crystal surface, which could form a protective layer and favor the formation of a smooth and dense solid electrolyte interphase with high toughness and Li+ ion conductivity. Therefore, the electrolyte system with 2.0 wt% 15‐C‐5 achieves excellent electrochemical performance with 170 cycles at 1.0 mA cm−2 with capacity of 0.5 mA h cm−2 in symmetric Li|Li cells. The obviously enhanced cycle and rate performance are also achieved in Li|LiNi 0.6 Co 0.2 Mn 0.2 O 2 (NCM622) full cells. The 15‐C‐5 demonstrates to be a promising additive for the electrolytes toward safe and efficient Li metal batteries.
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Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Fluoroethylene Carbonate Additives to Render Uniform Li Deposits in Lithium Metal Batteries
Zhang, X., Cheng, X., Chen, X., Yan, C., & Zhang, Q. (2017) · Advanced Functional Materials · doi:10.1002/adfm.201605989 · Cited by 1,699
Atomic structure of sensitive battery materials and interfaces revealed by cryo–electron microscopy
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Advanced Model for Solid Electrolyte Interphase Electrodes in Liquid and Polymer Electrolytes
Peled, E., Golodnitsky, D., & Ardel, G. (1997) · Journal of The Electrochemical Society · doi:10.1149/1.1837858 · Cited by 1,205
Identifying the components of the solid–electrolyte interphase in Li-ion batteries
Wang, L., Menakath, A., Han, F., Wang, Y., Zavalij, P. Y., Gaskell, K. J., Borodin, O., Iuga, D., Brown, S. P., Wang, C., et al. (2019) · Nature Chemistry · doi:10.1038/s41557-019-0304-z · Cited by 514
Cited by
Wu, D., He, J., Liu, J., Wu, M., Qi, S., Wang, H., Huang, J., Li, F., Tang, D., & Ma, J. (2022) · Advanced Energy Materials · doi:10.1002/aenm.202200337 · Cited by 319
Self-citationInsights into the deposition chemistry of Li ions in nonaqueous electrolyte for stable Li anodes
Wang, Z., Sun, Z., Li, J., Shi, Y., Sun, C., An, B., Cheng, H.-M., & Li, F. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01017k · Cited by 268
Wang, Z., Sun, Z., Shi, Y., Qi, F., Gao, X., Yang, H., Cheng, H., & Li, F. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202100935 · Cited by 202
Metadata
- Authors
- Wang, H., He, J., Liu, J., Qi, S., Wu, M., Wen, J., Chen, Y., Feng, Y., & Ma, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2020-07-12
- Volume
- 31
- Issue
- 2
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W3042414527
- Cited by
- 174
- References
- 5
- FWCI
- 8.86
- Type
- journal article
- Language
- en
- Open access
- closed
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