The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Toward a Low‐Cost Artificial Leaf: Driving Carbon‐Based and Bifunctional Catalyst Electrodes with Solution‐Processed Perovskite Photovoltaics
Open accessAbstract
Molecular hydrogen can be generated renewably by water splitting with an “artificial‐leaf device”, which essentially comprises two electrocatalyst electrodes immersed in water and powered by photovoltaics. Ideally, this device should operate efficiently and be fabricated with cost‐efficient means using earth‐abundant materials. Here, a lightweight electrocatalyst electrode, comprising large surface‐area NiCo 2 O 4 nanorods that are firmly anchored onto a carbon–paper current collector via a dense network of nitrogen‐doped carbon nanotubes is presented. This electrocatalyst electrode is bifunctional in that it can efficiently operate as both anode and cathode in the same alkaline solution, as quantified by a delivered current density of 10 mA cm−2 at an overpotential of 400 mV for each of the oxygen and hydrogen evolution reactions. By driving two such identical electrodes with a solution‐processed thin‐film perovskite photovoltaic assembly, a wired artificial‐leaf device is obtained that features a Faradaic H 2 evolution efficiency of 100%, and a solar‐to‐hydrogen conversion efficiency of 6.2%. A detailed cost analysis is presented, which implies that the material‐payback time of this device is of the order of 100 days.
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Cites
Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
Luo, J., Im, J.-H., Mayer, M. T., Schreier, M., Nazeeruddin, M. K., Park, N.-G., Tilley, S. D., Fan, H. J., & Grätzel, M. (2014) · Science · doi:10.1126/science.1258307 · Cited by 2,509
Toward the rational design of non-precious transition metal oxides for oxygen electrocatalysis
Hong, W. T., Risch, M., Stoerzinger, K. A., Grimaud, A., Suntivich, J., & Shao-Horn, Y. (2015) · Energy & Environmental Science · doi:10.1039/c4ee03869j · Cited by 2,089
Wang, H., Lee, H.-W., Deng, Y., Lu, Z., Hsu, P.-C., Liu, Y., Lin, D., & Cui, Y. (2015) · Nature Communications · doi:10.1038/ncomms8261 · Cited by 1,257
Ni–Mo Nanopowders for Efficient Electrochemical Hydrogen Evolution
McKone, J. R., Sadtler, B. F., Werlang, C. A., Lewis, N. S., & Gray, H. B. (2013) · ACS Catalysis · doi:10.1021/cs300691m · Cited by 798
Cui, X., Ren, P., Deng, D., Deng, J., & Bao, X. (2016) · Energy & Environmental Science · doi:10.1039/c5ee03316k · Cited by 791
Cited by
Advances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels
Birdja, Y. Y., Pérez-Gallent, E., Figueiredo, M. C., Göttle, A. J., Calle-Vallejo, F., & Koper, M. T. M. (2019) · Nature Energy · doi:10.1038/s41560-019-0450-y · Cited by 2,747
From Lithium‐Ion to Sodium‐Ion Batteries: Advantages, Challenges, and Surprises
Nayak, P. K., Yang, L., Brehm, W., & Adelhelm, P. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201703772 · Cited by 2,674
Wadsworth, A., Moser, M., Marks, A., Little, M. S., Gasparini, N., Brabec, C. J., Baran, D., & McCulloch, I. (2019) · Chemical Society Reviews · doi:10.1039/c7cs00892a · Cited by 986
Sodium‐Ion Battery Materials and Electrochemical Properties Reviewed
Chayambuka, K., Mulder, G., Danilov, D. L., & Notten, P. H. L. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201800079 · Cited by 733
Bresser, D., Buchholz, D., Moretti, A., Varzi, A., & Passerini, S. (2018) · Energy & Environmental Science · doi:10.1039/c8ee00640g · Cited by 640
Metadata
- Authors
- Sharifi, T., Larsen, C., Wang, J., Kwong, W. L., Gracia‐Espino, E., Mercier, G., Messinger, J., Wågberg, T., & Edman, L.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2016-07-19
- Volume
- 6
- Issue
- 20
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2503287062
- Cited by
- 639
- References
- 5
- FWCI
- 27.00
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Sharifi, T., Larsen, C., Wang, J., Kwong, W. L., Gracia‐Espino, E., Mercier, G., Messinger, J., Wågberg, T., & Edman, L. (2016). Toward a Low‐Cost Artificial Leaf: Driving Carbon‐Based and Bifunctional Catalyst Electrodes with Solution‐Processed Perovskite Photovoltaics. Advanced Energy Materials. https://doi.org/10.1002/aenm.201600738
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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