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Cited by 252

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Ruthenium Oxide Nanosheets for Enhanced Oxygen Evolution Catalysis in Acidic Medium

Open access
Laha, Sourav, Lee, Yonghyuk, Podjaski, Filip, Weber, Daniel, Duppel, Viola, Schoop, Leslie M., Pielnhofer, Florian, Scheurer, Christoph, Müller, Kathrin, Starke, Ulrich, Reuter, Karsten, Lotsch, Bettina V.·2019·Advanced Energy Materials

Abstract

The fabrication of highly active and robust hexagonal ruthenium oxide nanosheets for the electrocatalytic oxygen evolution reaction (OER) in an acidic environment is reported. The ruthenate nanosheets exhibit the best OER activity of all solution‐processed acid medium electrocatalysts reported to date, reaching 10 mA cm−2 at an overpotential of only ≈255 mV. The nanosheets also demonstrate robustness under harsh oxidizing conditions. Theoretical calculations give insights into the OER mechanism and reveal that the edges are the origin of the high OER activity of the nanosheets. Moreover, the post OER analyses indicate, apart from coarsening, no observable change in the morphology of the nanosheets or oxidation states of ruthenium during the electrocatalytic process. Therefore, the present investigation suggests that ruthenate nanosheets are a promising acid medium OER catalyst with application potential in proton exchange membrane electrolyzers and beyond.

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Metadata

Authors
Laha, S., Lee, Y., Podjaski, F., Weber, D., Duppel, V., Schoop, L. M., Pielnhofer, F., Scheurer, C., Müller, K., Starke, U., Reuter, K., & Lotsch, B. V.
Venue
Advanced Energy Materials
Publisher
Wiley
Published
2019-02-21
Volume
9
Issue
15
ISSN
  • 1614-6832 (ISSN-L)
  • 1614-6840
OpenAlex
W2917007993
Cited by
252
References
10
FWCI
6.60
Type
journal article
Language
en
Open access
green

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CoChat. (2026). Citation check: Ruthenium Oxide Nanosheets for Enhanced Oxygen Evolution Catalysis in Acidic Medium. https://app.cochat.ai/papers/10.1002/aenm.201803795
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Laha, S., Lee, Y., Podjaski, F., Weber, D., Duppel, V., Schoop, L. M., Pielnhofer, F., Scheurer, C., Müller, K., Starke, U., Reuter, K., & Lotsch, B. V. (2019). Ruthenium Oxide Nanosheets for Enhanced Oxygen Evolution Catalysis in Acidic Medium. Advanced Energy Materials. https://doi.org/10.1002/aenm.201803795

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