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Reactions at supercritical conditions: Applications and fundamentals
Abstract
Supercritical fluids posses properties that make them attractive as media for chemical reactions. Conducting chemical reactions at supercritical conditions affords opportunities to manipulate the reaction environment (solvent properties) by manipulating pressure, to enhance the solubilities of reactants and products, to eliminate interphase transport limitations on reaction rates, and to integrate reaction and separation unit operations. Supercritical conditions may be advantageous for reactions involved in fuels processing, biomass conversion, biocatalysis, homogeneous and heterogeneous catalysis, environmental control, polymerization, materials synthesis, and chemical synthesis. Moreover, supercritical fluids can be used profitably in fundamental chemical investigations of intermolecular interactions and their influence on chemical processes. Work on chemical reactions in and with supercritical fluids is reviewed. We discuss both fundamental studies and applications of reactions at supercritical conditions, with focus on work published after 1985.
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Cited by
Peterson, A. A., Vogel, F., Lachance, R. P., Fröling, M., Antal, Jr., & Tester, J. W. (2008) · Energy & Environmental Science · doi:10.1039/b810100k · Cited by 2,132
Roles of Water for Chemical Reactions in High-Temperature Water
Akiya, N., & Savage, P. E. (2002) · Chemical Reviews · doi:10.1021/cr000668w · Cited by 1,581
Self-citationA review on process conditions for optimum bio-oil yield in hydrothermal liquefaction of biomass
Akhtar, J., & Amin, N. A. S. (2011) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2010.11.054 · Cited by 1,059
Corrosion in high-temperature and supercritical water and aqueous solutions: a review
Kritzer, P. (2004) · The Journal of Supercritical Fluids · doi:10.1016/s0896-8446(03)00031-7 · Cited by 660
Valorization of hydrothermal liquefaction aqueous phase: pathways towards commercial viability
Watson, J., Wang, T., Si, B., Chen, W.-T., Aierzhati, A., & Zhang, Y. (2020) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2019.100819 · Cited by 394
Metadata
- Authors
- Savage, P. E., Gopalan, S., Mizan, T. I., Martino, C. J., & Brock, E. E.
- Venue
- AIChE Journal
- Publisher
- Wiley
- Published
- 1995-07
- Volume
- 41
- Issue
- 7
- Pages
- 1723-1778
- ISSN
- 0001-1541 (ISSN-L)
- 1547-5905
- OpenAlex
- W2153706306
- Cited by
- 945
- References
- 0
- FWCI
- 40.44
- Type
- journal article
- Language
- en
- Open access
- closed
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- Savage, P. E., Gopalan, S., Mizan, T. I., Martino, C. J., & Brock, E. E. (1995). Reactions at supercritical conditions: Applications and fundamentals. AIChE Journal. https://doi.org/10.1002/aic.690410712
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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