The DOI matches its Crossref record; 30 of the 30 references it cites were found in a registry or an index.
Sulfur Cathodes Based on Conductive MXene Nanosheets for High‐Performance Lithium–Sulfur Batteries
Abstract
Lithium–sulfur batteries are amongst the most promising candidates to satisfy emerging energy‐storage demands. Suppression of the polysulfide shuttle while maintaining high sulfur content is the main challenge that faces their practical development. Here, we report that 2D early‐transition‐metal carbide conductive MXene phases—reported to be impressive supercapacitor materials—also perform as excellent sulfur battery hosts owing to their inherently high underlying metallic conductivity and self‐functionalized surfaces. We show that 70 wt % S/Ti 2 C composites exhibit stable long‐term cycling performance because of strong interaction of the polysulfide species with the surface Ti atoms, demonstrated by X‐ray photoelectron spectroscopy studies. The cathodes show excellent cycling performance with specific capacity close to 1200 mA h g−1 at a five‐hour charge/discharge (C/5) current rate. Capacity retention of 80 % is achieved over 400 cycles at a two‐hour charge/discharge (C/2) current rate.
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Cites
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Two‐Dimensional Nanocrystals Produced by Exfoliation of Ti3AlC2
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25th Anniversary Article: MXenes: A New Family of Two‐Dimensional Materials
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Self-citationWhere do batteries end and supercapacitors begin?
Simon, P., Gogotsi, Y., & Dunn, B. (2014) · Science · doi:10.1126/science.1249625 · Cited by 5,634
Two-Dimensional Transition Metal Carbides
Naguib, M., Mashtalir, O., Carle, J., Presser, V., Lu, J., Hultman, L., Gogotsi, Y., & Barsoum, M. W. (2012) · ACS Nano · doi:10.1021/nn204153h · Cited by 4,769
Cation Intercalation and High Volumetric Capacitance of Two-Dimensional Titanium Carbide
Lukatskaya, M. R., Mashtalir, O., Ren, C. E., Dall’Agnese, Y., Rozier, P., Taberna, P. L., Naguib, M., Simon, P., Barsoum, M. W., & Gogotsi, Y. (2013) · Science · doi:10.1126/science.1241488 · Cited by 4,320
Intercalation and delamination of layered carbides and carbonitrides
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Polysulfide Shuttle Study in the Li/S Battery System
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Cited by
MXene chemistry, electrochemistry and energy storage applications
Li, X., Huang, Z., Shuck, C. E., Liang, G., Gogotsi, Y., & Zhi, C. (2022) · Nature Reviews Chemistry · doi:10.1038/s41570-022-00384-8 · Cited by 1,495
2D MXenes: A New Family of Promising Catalysts for the Hydrogen Evolution Reaction
Gao, G., O’Mullane, A. P., & Du, A. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b02754 · Cited by 1,153
A Two‐Dimensional Lamellar Membrane: MXene Nanosheet Stacks
Ding, L., Wei, Y., Wang, Y., Chen, H., Caro, J., & Wang, H. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201609306 · Cited by 1,111
High-entropy ceramics: Review of principles, production and applications
Akrami, S., Edalati, P., Fuji, M., & Edalati, K. (2021) · Materials Science and Engineering: R: Reports · doi:10.1016/j.mser.2021.100644 · Cited by 1,008
Zhao, S., Zhang, H.-B., Luo, J.-Q., Wang, Q.-W., Xu, B., Hong, S., & Yu, Z.-Z. (2018) · ACS Nano · doi:10.1021/acsnano.8b05739 · Cited by 893
Metadata
- Authors
- Liang, X., Garsuch, A., & Nazar, L. F.
- Venue
- Angewandte Chemie
- Publisher
- Wiley
- Published
- 2015-02-03
- Volume
- 127
- Issue
- 13
- Pages
- 3979-3983
- ISSN
- 0044-8249 (ISSN-L)
- 1521-3757
- OpenAlex
- W4250524647
- Cited by
- 313
- References
- 30
- FWCI
- 7.06
- Type
- journal article
- Language
- de
- Open access
- closed
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- Liang, X., Garsuch, A., & Nazar, L. F. (2015). Sulfur Cathodes Based on Conductive MXene Nanosheets for High‐Performance Lithium–Sulfur Batteries. Angewandte Chemie. https://doi.org/10.1002/ange.201410174
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