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Cobalt‐Based Complexes for the Copolymerization of Propylene Oxide and CO2: Active and Selective Catalysts for Polycarbonate Synthesis
Open accessAbstract
CO2 is an ideal feedstock for chemical synthesis; unfortunately its thermodynamic stability is a barrier to widespread use. Active cobalt catalysts for the copolymerization of propylene oxide and CO2 are reported (see scheme; L=N,N′-bis(3,5-di-tert-butylsalicylidene)-1,2-cyclohexanediamine), which have excellent regioselectivity for polycarbonate synthesis without concomitant production of cyclic carbonate by-products.
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Citations
Cites
Polymerization of lactide and related cyclic esters by discrete metal complexes
O'Keefe, B. J., Hillmyer, M. A., & Tolman, W. B. (2001) · Journal of the Chemical Society, Dalton Transactions · doi:10.1039/b104197p · Cited by 825
Cited by
Darensbourg, D. J. (2007) · Chemical Reviews · doi:10.1021/cr068363q · Cited by 1,593
Coates, G. W., & Moore, D. R. (2004) · Angewandte Chemie International Edition · doi:10.1002/anie.200460442 · Cited by 1,154
Self-citationCatalysts for CO 2 /epoxide copolymerisation
Kember, M. R., Buchard, A., & Williams, C. K. (2011) · Chem. Commun. · doi:10.1039/c0cc02207a · Cited by 797
Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer
Xie, Y., Wang, T.-T., Liu, X.-H., Zou, K., & Deng, W.-Q. (2013) · Nature Communications · doi:10.1038/ncomms2960 · Cited by 772
Recent advances in CO2/epoxide copolymerization—New strategies and cooperative mechanisms
Klaus, S., Lehenmeier, M. W., Anderson, C. E., & Rieger, B. (2011) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2010.12.002 · Cited by 710
Metadata
- Authors
- Qin, Z., Thomas, C. M., Lee, S., & Coates, G. W.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2003-11-11
- Volume
- 42
- Issue
- 44
- Pages
- 5484-5487
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2155632989
- Cited by
- 415
- References
- 1
- FWCI
- 12.72
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Qin, Z., Thomas, C. M., Lee, S., & Coates, G. W. (2003). Cobalt‐Based Complexes for the Copolymerization of Propylene Oxide and CO2: Active and Selective Catalysts for Polycarbonate Synthesis. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200352605
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