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Highly Active, Binary Catalyst Systems for the Alternating Copolymerization of CO2 and Epoxides under Mild Conditions
Open accessAbstract
Excellent activity and selectivity in the copolymerization of CO2 with epoxides at extremely mild temperature and pressure are observed in the presence of binary nucleophile–electrophile catalyst systems based on chiral [(salcy)CoIIIX] complexes and quaternary ammonium salts (see scheme). Completely alternating copolymers are obtained with >95 % head-to-tail linkages.
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Citations
Cites
Asymmetric Catalysis of Epoxide Ring-Opening Reactions
Jacobsen, E. N. (2000) · Accounts of Chemical Research · doi:10.1021/ar960061v · Cited by 1,261
Cited by
Darensbourg, D. J. (2007) · Chemical Reviews · doi:10.1021/cr068363q · Cited by 1,593
Catalysts for CO 2 /epoxide copolymerisation
Kember, M. R., Buchard, A., & Williams, C. K. (2011) · Chem. Commun. · doi:10.1039/c0cc02207a · Cited by 797
Recent advances in CO2/epoxide copolymerization—New strategies and cooperative mechanisms
Klaus, S., Lehenmeier, M. W., Anderson, C. E., & Rieger, B. (2011) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2010.12.002 · Cited by 710
Ring-opening copolymerization (ROCOP): synthesis and properties of polyesters and polycarbonates
Paul, S., Zhu, Y., Romain, C., Brooks, R., Saini, P. K., & Williams, C. K. (2015) · Chemical Communications · doi:10.1039/c4cc10113h · Cited by 593
Stereoselective Epoxide Polymerization and Copolymerization
Childers, M. I., Longo, J. M., Van Zee, N. J., LaPointe, A. M., & Coates, G. W. (2014) · Chemical Reviews · doi:10.1021/cr400725x · Cited by 471
Metadata
- Authors
- Lu, X., & Wang, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2004-06-29
- Volume
- 43
- Issue
- 27
- Pages
- 3574-3577
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2017589181
- Cited by
- 346
- References
- 1
- FWCI
- 14.01
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Lu, X., & Wang, Y. (2004). Highly Active, Binary Catalyst Systems for the Alternating Copolymerization of CO2 and Epoxides under Mild Conditions. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200453998
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
