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Oxidative Dehydrogenation on Nanocarbon: Identification and Quantification of Active Sites by Chemical Titration
Abstract
Ketonic carbonyl groups are catalytic active sites for oxidative dehydrogenation (ODH) reactions on carbon nanotubes. The quantity of these groups could be calculated from chemical titration with hydrazine compounds. ODH catalytic activity of nanocarbon is directly correlated with surface concentration of ketonic carbonyl groups, and the turnover frequency normalized by the number of active sites reflects the intrinsic activity of nanocarbon catalysts.
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Cited by
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Duan, X., Xu, J., Wei, Z., Ma, J., Guo, S., Wang, S., Liu, H., & Dou, S. (2017) · Advanced Materials · doi:10.1002/adma.201701784 · Cited by 754
Liang, J., Zhou, R. F., Chen, X. M., Tang, Y. H., & Qiao, S. Z. (2014) · Advanced Materials · doi:10.1002/adma.201401848 · Cited by 522
Unveiling the active sites of graphene-catalyzed peroxymonosulfate activation
Duan, X., Sun, H., Ao, Z., Zhou, L., Wang, G., & Wang, S. (2016) · Carbon · doi:10.1016/j.carbon.2016.06.016 · Cited by 498
Metadata
- Authors
- Qi, W., Liu, W., Zhang, B., Gu, X., Guo, X., & Su, D.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2013-11-08
- Volume
- 52
- Issue
- 52
- Pages
- 14224-14228
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2156948146
- Cited by
- 301
- References
- 0
- FWCI
- 7.12
- Type
- journal article
- Language
- en
- Open access
- closed
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- Qi, W., Liu, W., Zhang, B., Gu, X., Guo, X., & Su, D. (2013). Oxidative Dehydrogenation on Nanocarbon: Identification and Quantification of Active Sites by Chemical Titration. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201306825
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