The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Indium Oxide as a Superior Catalyst for Methanol Synthesis by CO2 Hydrogenation
Abstract
Methanol synthesis by CO 2 hydrogenation is attractive in view of avoiding the environmental implications associated with the production of the traditional syngas feedstock and mitigating global warming. However, there still is a lack of efficient catalysts for such alternative processes. Herein, we unveil the high activity, 100 % selectivity, and remarkable stability for 1000 h on stream of In 2 O 3 supported on ZrO 2 under industrially relevant conditions. This strongly contrasts to the benchmark Cu‐ZnO‐Al 2 O 3 catalyst, which is unselective and experiences rapid deactivation. In‐depth characterization of the In 2 O 3‐based materials points towards a mechanism rooted in the creation and annihilation of oxygen vacancies as active sites, whose amount can be modulated in situ by co‐feeding CO and boosted through electronic interactions with the zirconia carrier. These results constitute a promising basis for the design of a prospective technology for sustainable methanol production.
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Citations
Cites
Recent advances in catalytic hydrogenation of carbon dioxide
Wang, W., Wang, S., Ma, X., & Gong, J. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15008a · Cited by 3,316
Cited by
Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Tuning Selectivity of CO2 Hydrogenation Reactions at the Metal/Oxide Interface
Kattel, S., Liu, P., & Chen, J. G. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b05362 · Cited by 1,259
Direct conversion of CO2 into liquid fuels with high selectivity over a bifunctional catalyst
Gao, P., Li, S., Bu, X., Dang, S., Liu, Z., Wang, H., Zhong, L., Qiu, M., Yang, C., Cai, J., et al. (2017) · Nature Chemistry · doi:10.1038/nchem.2794 · Cited by 1,122
Zhang, L., Zhao, Z., & Gong, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201612214 · Cited by 1,048
Direct Production of Lower Olefins from CO2 Conversion via Bifunctional Catalysis
Gao, P., Dang, S., Li, S., Bu, X., Liu, Z., Qiu, M., Yang, C., Wang, H., Zhong, L., Han, Y., et al. (2018) · ACS Catalysis · doi:10.1021/acscatal.7b02649 · Cited by 533
Metadata
- Authors
- Martin, O., Martín, A. J., Mondelli, C., Mitchell, S., Segawa, T. F., Hauert, R., Drouilly, C., Curulla‐Ferré, D., & Pérez‐Ramírez, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-03-17
- Volume
- 55
- Issue
- 21
- Pages
- 6261-6265
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2300085411
- Cited by
- 1,119
- References
- 1
- FWCI
- 20.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Martin, O., Martín, A. J., Mondelli, C., Mitchell, S., Segawa, T. F., Hauert, R., Drouilly, C., Curulla‐Ferré, D., & Pérez‐Ramírez, J. (2016). Indium Oxide as a Superior Catalyst for Methanol Synthesis by CO2 Hydrogenation. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201600943
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