The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Highly Efficient CO2 Electroreduction on ZnN4‐based Single‐Atom Catalyst
Abstract
The electrochemical reduction reaction of carbon dioxide (CO2RR) to carbon monoxide (CO) is the basis for the further synthesis of more complex carbon‐based fuels or attractive feedstock. Single‐atom catalysts have unique electronic and geometric structures with respect to their bulk counterparts, thus exhibiting unexpected catalytic activities. A nitrogen‐anchored Zn single‐atom catalyst is presented for CO formation from CO2RR with high catalytic activity (onset overpotential down to 24 mV), high selectivity (Faradaic efficiency for CO (FE CO) up to 95 % at −0.43 V), remarkable durability (>75 h without decay of FE CO), and large turnover frequency (TOF, up to 9969 h−1). Further experimental and DFT results indicate that the four‐nitrogen‐anchored Zn single atom (Zn‐N 4) is the main active site for CO2RR with low free energy barrier for the formation of *COOH as the rate‐limiting step.
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Cites
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
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Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
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Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
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Ionic Liquid–Mediated Selective Conversion of CO 2 to CO at Low Overpotentials
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High performance platinum single atom electrocatalyst for oxygen reduction reaction
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Self-citationTuning of CO2 Reduction Selectivity on Metal Electrocatalysts
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Nitrogen-Based Catalysts for the Electrochemical Reduction of CO 2 to CO
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
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Single atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
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Stable and Efficient Single-Atom Zn Catalyst for CO2 Reduction to CH4
Han, L., Song, S., Liu, M., Yao, S., Liang, Z., Cheng, H., Ren, Z., Liu, W., Lin, R., Qi, G., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b12111 · Cited by 538
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Metadata
- Authors
- Yang, F., Song, P., Liu, X., Mei, B., Xing, W., Jiang, Z., Gu, L., & Xu, W.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-08-23
- Volume
- 57
- Issue
- 38
- Pages
- 12303-12307
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2883032287
- Cited by
- 456
- References
- 10
- FWCI
- 11.82
- Type
- journal article
- Language
- en
- Open access
- closed
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