The DOI matches its Crossref record; 23 of the 23 references it cites were found in a registry or an index.
Paired Electrocatalytic Oxygenation and Hydrogenation of Organic Substrates with Water as the Oxygen and Hydrogen Source
Open accessAbstract
The use of water as an oxygen and hydrogen source for the paired oxygenation and hydrogenation of organic substrates to produce valuable chemicals is of utmost importance as a means of establishing green chemical syntheses. Inspired by the active Ni 3+ intermediates involved in electrocatalytic water oxidation by nickel‐based materials, we prepared NiBx as a catalyst and used water as the oxygen source for the oxygenation of various organic compounds. NiBx was further employed as both an anode and a cathode in a paired electrosynthesis cell for the respective oxygenation and hydrogenation of organic compounds, with water as both the oxygen and hydrogen source. Conversion efficiency and selectivity of ≥99 % were observed during the oxygenation of 5‐hydroxymethylfurfural to 2,5‐furandicarboxylic acid and the simultaneous hydrogenation of p‐nitrophenol to p‐aminophenol. This paired electrosynthesis cell has also been coupled to a solar cell as a stand‐alone reactor in response to sunlight.
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Synthetic Organic Electrochemical Methods Since 2000: On the Verge of a Renaissance
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New interpretations of XPS spectra of nickel metal and oxides
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Modern Electrochemical Aspects for the Synthesis of Value‐Added Organic Products
Möhle, S., Zirbes, M., Rodrigo, E., Gieshoff, T., Wiebe, A., & Waldvogel, S. R. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201712732 · Cited by 1,098
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Catalytic oxidation of carbohydrates into organic acids and furan chemicals
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Cited by
Yang, Y., & Mu, T. (2021) · Green Chemistry · doi:10.1039/d1gc00914a · Cited by 539
Electrochemical hydrogenation and oxidation of organic species involving water
Liu, C., Chen, F., Zhao, B.-H., Wu, Y., & Zhang, B. (2024) · Nature Reviews Chemistry · doi:10.1038/s41570-024-00589-z · Cited by 269
Self-citationChen, D., Ding, Y., Cao, X., Wang, L., Lee, H., Lin, G., Li, W., Ding, G., & Sun, L. (2023) · Angewandte Chemie International Edition · doi:10.1002/anie.202309478 · Cited by 235
Self-citationActivated Ni–OH Bonds in a Catalyst Facilitates the Nucleophile Oxidation Reaction
Chen, W., Wang, Y., Wu, B., Shi, J., Li, Y., Xu, L., Xie, C., Zhou, W., Huang, Y., Wang, T., et al. (2022) · Advanced Materials · doi:10.1002/adma.202105320 · Cited by 200
Bharath, G., Rambabu, K., Hai, A., Banat, F., Taher, H., Schmidt, J. E., & Show, P. L. (2020) · Energy Conversion and Management · doi:10.1016/j.enconman.2020.112859 · Cited by 70
Metadata
- Authors
- Zhang, P., Sheng, X., Chen, X., Fang, Z., Jiang, J., Wang, M., Li, F., Fan, L., Ren, Y., Zhang, B., Timmer, B. J. J., Ahlquist, M. S. G., & Sun, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-05-22
- Volume
- 58
- Issue
- 27
- Pages
- 9155-9159
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2942186791
- Cited by
- 298
- References
- 23
- FWCI
- 7.01
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Zhang, P., Sheng, X., Chen, X., Fang, Z., Jiang, J., Wang, M., Li, F., Fan, L., Ren, Y., Zhang, B., Timmer, B. J. J., Ahlquist, M. S. G., & Sun, L. (2019). Paired Electrocatalytic Oxygenation and Hydrogenation of Organic Substrates with Water as the Oxygen and Hydrogen Source. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201903936
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