The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
Electrochemical Oxidation of 5-Hydroxymethylfurfural with NiFe Layered Double Hydroxide (LDH) Nanosheet Catalysts
Abstract
Electrochemical oxidation of biomass-derived platform molecules can enable the production of value-added oxygenated commodity chemicals under mild conditions in a distributed fashion using renewable electricity; however, very few efficient, robust, and inexpensive electrocatalysts are available for such electrochemical oxidation. Here we demonstrate that earth-abundant NiFe layered double hydroxide (LDH) nanosheets grown on carbon fiber paper can efficiently catalyze the oxidation of 5-hydroxymethylfurfural (HMF) to 2,5-furandicarboxylic acid (FDCA) at the anode of an electrochemical cell. A near-quantitative yield of FDCA and 99.4% Faradaic efficiency of HMF conversion under ambient conditions can be achieved in the electrochemical process. HMF has a higher rate of oxidation than water and can act as an alternative anodic reaction for alkaline H 2 evolution in water-splitting cells. As the first report on using bimetallic metal hydroxide/oxide catalysts for electrochemical oxidation of HMF, this work opens up opportunities in electrochemical devices to simultaneously produce building-block chemicals from biomass-derived molecules and clean H 2 fuels under ambient conditions with earth-abundant materials.
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Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
Bozell, J. J., & Petersen, G. R. (2010) · Green Chemistry · doi:10.1039/b922014c · Cited by 4,566
Hydroxymethylfurfural, A Versatile Platform Chemical Made from Renewable Resources
van Putten, R.-J., van der Waal, J. C., de Jong, E., Rasrendra, C. B., Heeres, H. J., & de Vries, J. G. (2013) · Chemical Reviews · doi:10.1021/cr300182k · Cited by 2,886
Homogeneously dispersed multimetal oxygen-evolving catalysts
Zhang, B., Zheng, X., Voznyy, O., Comin, R., Bajdich, M., García-Melchor, M., Han, L., Xu, J., Liu, M., Zheng, L., et al. (2016) · Science · doi:10.1126/science.aaf1525 · Cited by 2,447
Faber, M. S., & Jin, S. (2014) · Energy Environ. Sci. · doi:10.1039/c4ee01760a · Cited by 1,317
Self-citationZhu, J., Cai, J., Xie, W., Chen, P.-H., Gazzano, M., Scandola, M., & Gross, R. A. (2013) · Macromolecules · doi:10.1021/ma3023298 · Cited by 333
Cited by
Yang, Y., & Mu, T. (2021) · Green Chemistry · doi:10.1039/d1gc00914a · Cited by 539
Zhang, N., Zou, Y., Tao, L., Chen, W., Zhou, L., Liu, Z., Zhou, B., Huang, G., Lin, H., & Wang, S. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201908722 · Cited by 523
Electrocatalytic Oxidation of 5‐(Hydroxymethyl)furfural Using High‐Surface‐Area Nickel Boride
Barwe, S., Weidner, J., Cychy, S., Morales, D. M., Dieckhöfer, S., Hiltrop, D., Masa, J., Muhler, M., & Schuhmann, W. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201806298 · Cited by 507
Han, X., Sheng, H., Yu, C., Walker, T. W., Huber, G. W., Qiu, J., & Jin, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01498 · Cited by 445
Self-citationIglesias, J., Martínez-Salazar, I., Maireles-Torres, P., Martin Alonso, D., Mariscal, R., & López Granados, M. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00177e · Cited by 292
Metadata
- Authors
- Liu, W.-J., Dang, L., Xu, Z., Yu, H.-Q., Jin, S., & Huber, G. W.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-05-10
- Volume
- 8
- Issue
- 6
- Pages
- 5533-5541
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2801231312
- Cited by
- 507
- References
- 6
- FWCI
- 16.04
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, W.-J., Dang, L., Xu, Z., Yu, H.-Q., Jin, S., & Huber, G. W. (2018). Electrochemical Oxidation of 5-Hydroxymethylfurfural with NiFe Layered Double Hydroxide (LDH) Nanosheet Catalysts. ACS Catalysis. https://doi.org/10.1021/acscatal.8b01017
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