Cited by 426Aqueous and Flow BatteriesAdvancements in Battery MaterialsAdvanced Battery Materials and Technologies

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Aqueous Batteries Operated at −50 °C

Nian, Qingshun, Wang, Jiayue, Liu, Shuang, Sun, Tianjiang, Zheng, Shibing, Zhang, Yan, Tao, Zhanliang, Chen, Jun·2019·Angewandte Chemie International Edition

DOI 10.1002/anie.201908913

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Abstract

Insufficient ionic conductivity and freezing of the electrolyte are considered the main problems for electrochemical energy storage at low temperatures (low T). Here, an electrolyte with a freezing point lower than −130 °C is developed by using dimethyl sulfoxide (DMSO) as an additive with molar fraction of 0.3 to an aqueous solution of 2 m NaClO 4 (2M‐0.3 electrolyte). The 2M‐0.3 electrolyte exhibits sufficient ionic conductivity of 0.11 mS cm −1 at −50 °C. The combination of spectroscopic investigations and molecular dynamics (MD) simulations reveal that hydrogen bonds are stably formed between DMSO and water molecules, facilitating the operation of the electrolyte at ultra‐low T. Using DMSO as the electrolyte additive, the aqueous rechargeable alkali‐ion batteries (AABs) can work well even at −50 °C. This work provides a simple and effective strategy to develop low T AABs.

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Authors: Nian, Q., Wang, J., Liu, S., Sun, T., Zheng, S., Zhang, Y., Tao, Z., & Chen, J.
Affiliations: Nankai University (CN)
Dalian Institute of Chemical Physics (CN)
Shandong University (CN)
Corresponding author: Tao, Zhanliang
ORCID: Nian, Qingshun
Wang, Jiayue
Liu, Shuang
Tao, Zhanliang
Chen, Jun
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2019-10-15
Volume: 58
Issue: 47
Pages: 16994-16999
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.201908913
OpenAlex: W2974348764
Cited by: 426
References: 0
Citations by year: 2026: 32 · 2025: 59 · 2024: 99 · 2023: 70 · 2022: 74 · 2021: 59 · 2020: 32 · 2019: 1
FWCI: 2.10
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
PubMed (publishedVersion)
Funders: National Natural Science Foundation of China (51771094,21835004)
Ministry of Education (B12015 and IRT13R30)
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Aqueous and Flow Batteries
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
Keywords: aqueous batteries, low-temperature batteries, NaClO4 electrolyte, ionic conductivity, hydrogen bonding, alkali-ion batteries, molecular dynamics simulation, electrochemical energy storage

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