The DOI matches its Crossref record; 36 of the 36 references it cites were found in a registry or an index.
Dynamic Activation of Adsorbed Intermediates via Axial Traction for the Promoted Electrochemical CO2 Reduction
Abstract
Regulating the local environment and structure of metal center coordinated by nitrogen ligands (M‐N 4) to accelerate overall reaction dynamics of the electrochemical CO 2 reduction reaction (CO 2 RR) has attracted extensive attention. Herein, we develop an axial traction strategy to optimize the electronic structure of the M‐N 4 moiety and construct atomically dispersed nickel sites coordinated with four nitrogen atoms and one axial oxygen atom, which are embedded within the carbon matrix (Ni‐N 4‐O/C). The Ni‐N 4‐O/C electrocatalyst exhibited excellent CO 2 RR performance with a maximum CO Faradic efficiency (FE) close to 100 % at −0.9 V. The CO FE could be maintained above 90 % in a wide range of potential window from −0.5 to −1.1 V. The superior CO 2 RR activity is due to the Ni‐N 4‐O active moiety composed of a Ni‐N 4 site with an additional oxygen atom that induces an axial traction effect.
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Cites
Single-Atom Catalysts: Synthetic Strategies and Electrochemical Applications
Chen, Y., Ji, S., Chen, C., Peng, Q., Wang, D., & Li, Y. (2018) · Joule · doi:10.1016/j.joule.2018.06.019 · Cited by 2,258
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
Atomically dispersed manganese catalysts for oxygen reduction in proton-exchange membrane fuel cells
Li, J., Chen, M., Cullen, D. A., Hwang, S., Wang, M., Li, B., Liu, K., Karakalos, S., Lucero, M., Zhang, H., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0164-8 · Cited by 1,496
Self-citationYuan, K., Lützenkirchen-Hecht, D., Li, L., Shuai, L., Li, Y., Cao, R., Qiu, M., Zhuang, X., Leung, M. K. H., Chen, Y., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b11852 · Cited by 1,047
Self-citationAdvanced Electrocatalysts with Single-Metal-Atom Active Sites
Wang, Y., Su, H., He, Y., Li, L., Zhu, S., Shen, H., Xie, P., Fu, X., Zhou, G., Feng, C., et al. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00594 · Cited by 1,005
Self-citationHuang, L., Chen, J., Gan, L., Wang, J., & Dong, S. (2019) · Science Advances · doi:10.1126/sciadv.aav5490 · Cited by 993
Self-citationExclusive Ni–N4 Sites Realize Near-Unity CO Selectivity for Electrochemical CO2 Reduction
Li, X., Bi, W., Chen, M., Sun, Y., Ju, H., Yan, W., Zhu, J., Wu, X., Chu, W., Wu, C., et al. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b09074 · Cited by 932
Jiang, R., Li, L., Sheng, T., Hu, G., Chen, Y., & Wang, L. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b07294 · Cited by 797
He, Y., Liu, S., Priest, C., Shi, Q., & Wu, G. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00903e · Cited by 771
Self-citationCoordinatively unsaturated nickel–nitrogen sites towards selective and high-rate CO2electroreduction
Yan, C., Li, H., Ye, Y., Wu, H., Cai, F., Si, R., Xiao, J., Miao, S., Xie, S., Yang, F., et al. (2018) · Energy & Environmental Science · doi:10.1039/c8ee00133b · Cited by 768
Cited by
Tang, T., Wang, Z., & Guan, J. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202111504 · Cited by 304
Wang, X., Sang, X., Dong, C., Yao, S., Shuai, L., Lu, J., Yang, B., Li, Z., Lei, L., Qiu, M., et al. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202100011 · Cited by 267
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Metadata
- Authors
- Wang, X., Wang, Y., Sang, X., Zheng, W., Zhang, S., Shuai, L., Yang, B., Li, Z., Chen, J., Lei, L., Adli, N. M., Leung, M. K. H., Qiu, M., Wu, G., & Hou, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-01-29
- Volume
- 60
- Issue
- 8
- Pages
- 4192-4198
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3104917636
- Cited by
- 294
- References
- 36
- FWCI
- 8.43
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, X., Wang, Y., Sang, X., Zheng, W., Zhang, S., Shuai, L., Yang, B., Li, Z., Chen, J., Lei, L., Adli, N. M., Leung, M. K. H., Qiu, M., Wu, G., & Hou, Y. (2021). Dynamic Activation of Adsorbed Intermediates via Axial Traction for the Promoted Electrochemical CO2 Reduction. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202013427
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