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Near‐Infrared Light‐Driven Shape‐Morphing of Programmable Anisotropic Hydrogels Enabled by MXene Nanosheets

Xue, Pan, Bisoyi, Hari Krishna, Chen, Yuanhao, Zeng, Hao, Yang, Jiajia, Yang, Xiao, Lv, Pengfei, Zhang, Xinmu, Priimagi, Arri, Wang, Ling, Xu, Xinhua, Li, Quan·2021·Angewandte Chemie International Edition

Abstract

Herein, we report near‐infrared (NIR) light‐driven shape‐morphing of programmable MXene‐containing anisotropic hydrogel actuators that are fabricated through in situ free‐radical copolymerization of a judiciously designed MXene nanomonomer with thermosensitive hydrogel network. A low electric field (few V mm−1) was found to enable a spatial distribution of MXene nanosheets and hence introduce anisotropy into the hydrogel network. Programmable anisotropic hydrogel actuators were developed by controlling ITO electrode pattern, direct‐current (DC) electric field direction and mask‐assisted photopolymerization. As a proof‐of‐concept, we demonstrate NIR light‐driven shape morphing of the MXene‐containing anisotropic hydrogel into various shapes and devise a four‐arm soft gripper that can perform distinct photomechanical functions such as grasping, lifting/lowering down and releasing an object upon sequential NIR light exposure.

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Metadata

Authors
Xue, P., Bisoyi, H. K., Chen, Y., Zeng, H., Yang, J., Yang, X., Lv, P., Zhang, X., Priimagi, A., Wang, L., Xu, X., & Li, Q.
Venue
Angewandte Chemie International Edition
Publisher
Wiley
Published
2021-01-14
Volume
60
Issue
7
Pages
3390-3396
ISSN
  • 1433-7851 (ISSN-L)
  • 1521-3773
OpenAlex
W3107540151
Cited by
363
References
54
FWCI
24.61
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Near‐Infrared Light‐Driven Shape‐Morphing of Programmable Anisotropic Hydrogels Enabled by MXene Nanosheets. https://app.cochat.ai/papers/10.1002/anie.202014533
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Xue, P., Bisoyi, H. K., Chen, Y., Zeng, H., Yang, J., Yang, X., Lv, P., Zhang, X., Priimagi, A., Wang, L., Xu, X., & Li, Q. (2021). Near‐Infrared Light‐Driven Shape‐Morphing of Programmable Anisotropic Hydrogels Enabled by MXene Nanosheets. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202014533

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