Nuclear-based hydrogen production with a thermochemical copper-chlorine cycle and supercritical water reactor: equipment scale-up and process simulation
Open accessAbstract
Issues related to equipment scale-up and process simulation are described for a thermochemical cycle driven by nuclear heat from Canada's proposed Generation IV reactor (Super-Critical Water-Cooled Reactor; SCWR), which is a CANDU derivative using supercritical water cooling. The copper–chlorine (Cu-Cl) cycle has been identified by Atomic Energy of Canada Limited as the most promising cycle for thermochemical hydrogen production with SCWR. Water is decomposed into hydrogen and oxygen through intermediate Cu-Cl compounds. This article outlines the challenges and design issues of hydrogen production with a Cu-Cl cycle coupled to Canada's nuclear reactors. The processes are simulated using the Aspen Plus process simulation code, allowing the cycle efficiency and possible efficiency improvements to be examined. The results are useful to assist the development of a lab-scale cycle demonstration, which is currently being undertaken at the University of Ontario Institute of Technology in collaboration with numerous partners. Copyright © 2010 John Wiley & Sons, Ltd.
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This integration leads to higher efficiency, lower environmental influence, and lower expenses.
“This integration leads to higher efficiency, lower environmental influence, and lower expenses.175,333”
From Strategies To Improve the Performance of Hydrogen Storage Systems by Liquefaction Methods: A Comprehensive Review (2023) · cites this paper as [333]
The Discussion says using nuclear waste heat improves the cycle’s overall efficiency, and the Simulation results say the process could eliminate greenhouse-gas emissions. But those results also say its efficiency is currently lower than SMR’s and that costs may fall eventually; they do not establish that the integration already delivers lower expenses. (LLM, conf=0.88)
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Self-citation
- Authors
- Rosen, M. A., Naterer, G. F., Chukwu, C. C., Sadhankar, R., & Suppiah, S.
- Affiliations
- Ontario Tech University (CA)
- Atomic Energy (Canada) (CA)
- Corresponding author
- Rosen, M. A.
- Venue
- International Journal of Energy Research
- Publisher
- Hindawi Limited
- Published
- 2010-04-20
- Volume
- 36
- Issue
- 4
- Pages
- 456-465
- ISSN
- 0363-907X (ISSN-L)
- OpenAlex
- W2122885484
- Cited by
- 84
- References
- 45
- Citations by year
- 2026: 2 · 2025: 3 · 2024: 4 · 2023: 5 · 2022: 1 · 2021: 7 · 2020: 4 · 2019: 5 · 2018: 2 · 2017: 3 · 2016: 3 · 2015: 1 · 2014: 8 · 2013: 6 · 2012: 12
- FWCI
- 5.67
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- International Journal of Energy Research (publishedVersion)
- Funders
- Atomic Energy of Canada Limited
- Topics
- Physical Sciences › Engineering › Biomedical Engineering › Chemical Looping and Thermochemical Processes
- Physical Sciences › Engineering › Aerospace Engineering › Nuclear reactor physics and engineering
- Physical Sciences › Materials Science › Materials Chemistry › Nuclear Materials and Properties
- Keywords
- thermochemical hydrogen production, copper-chlorine cycle, supercritical water-cooled reactor, nuclear heat, process simulation, cycle efficiency, water splitting, Generation IV reactors, CANDU reactors, hydrogen production
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