Cited by 304Hydrogels: synthesis, properties, applicationsAdvanced Materials and MechanicsPolymer composites and self-healing

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pH-induced shape-memory polymers

Han, Xiao‐Juan, Dong, Zhen‐Qiang, Fan, Min‐Min, Liu, Yan, li, Jian‐Hu, Wang, Yi‐Fu, Yuan, Qi‐Juan, Li, Bang‐Jing, Zhang, Sheng·2012·Macromolecular Rapid Communications

DOI 10.1002/marc.201200153

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Abstract

A novel pH sensitive shape-memory polymer (SMP) is prepared by cross-linking the β-cyclodextrin modified alginate (β-CD-Alg) and diethylenetriamine modified alginate (DETA-Alg): The pH reversible β-CD-DETA inclusion complexes serve as a reversible phase, and the cross-linked alginate chains serve as a fixing phase. It is shown that this material can be processed into temporary shape as we needs at pH 11.5 and recover to its initial shape at pH 7. The recovery ratio and the fixity ratio were 95.7 ± 0.9% and 94.8 ± 1.1%, respectively. Furthermore, this material showed good degradability and biocompatibility. Because the shape transition pH value is quite close to that of our body fluid and this pH triggered shape-memory effect is convenient and safe to use, this material has a high potential for medical application.

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Authors: Han, X., Dong, Z., Fan, M., Liu, Y., li, J., Wang, Y., Yuan, Q., Li, B., & Zhang, S.
Affiliations: Sichuan University (CN)
Chinese Academy of Sciences (CN)
Corresponding author: Li, Bang‐Jing
Zhang, Sheng
ORCID: Liu, Yan
Li, Bang‐Jing
Zhang, Sheng
Venue: Macromolecular Rapid Communications
Publisher: Wiley
Published: 2012-04-20
Volume: 33
Issue: 12
Pages: 1055-1060
ISSN: 1022-1336 (ISSN-L)
1521-3927
DOI: 10.1002/marc.201200153
OpenAlex: W1981343413
Cited by: 304
References: 22
Citations by year: 2026: 10 · 2025: 21 · 2024: 22 · 2023: 23 · 2022: 20 · 2021: 37 · 2020: 33 · 2019: 27 · 2018: 31 · 2017: 16 · 2016: 20 · 2015: 16 · 2014: 12 · 2013: 13 · 2012: 3
FWCI: 6.46
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Macromolecular Rapid Communications (publishedVersion)
PubMed (publishedVersion)
Topics: Physical Sciences › Materials Science › Biomaterials › Hydrogels: synthesis, properties, applications
Physical Sciences › Engineering › Mechanical Engineering › Advanced Materials and Mechanics
Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
Keywords: shape memory polymers, pH-responsive materials, β-cyclodextrin, alginate, diethylenetriamine, inclusion complexes, shape recovery, biodegradability, biocompatibility, medical applications
MeSH terms: Alginates, Biocompatible Materials, Cross-Linking Reagents, Hydrogen-Ion Concentration, Polymers, Temperature, beta-Cyclodextrins

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