The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
High‐Performance Perovskite Composite Electrocatalysts Enabled by Controllable Interface Engineering
Abstract
Single‐phase perovskite oxides that contain nonprecious metals have long been pursued as candidates for catalyzing the oxygen evolution reaction, but their catalytic activity cannot meet the requirements for practical electrochemical energy conversion technologies. Here a cation deficiency‐promoted phase separation strategy to design perovskite‐based composites with significantly enhanced water oxidation kinetics compared to single‐phase counterparts is reported. These composites, self‐assembled from perovskite precursors, comprise strongly interacting perovskite and related phases, whose structure, composition, and concentration can be accurately controlled by tailoring the stoichiometry of the precursors. The composite catalyst with optimized phase composition and concentration outperforms known perovskite oxide systems and state‐of‐the‐art catalysts by 1–3 orders of magnitude. It is further demonstrated that the strong interfacial interaction of the composite catalysts plays a key role in promoting oxygen ionic transport to boost the lattice‐oxygen participated water oxidation. These results suggest a simple and viable approach to developing high‐performance, perovskite‐based composite catalysts for electrochemical energy conversion.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
Suen, N.-T., Hung, S.-F., Quan, Q., Zhang, N., Xu, Y.-J., & Chen, H. M. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00328a · Cited by 6,307
Homogeneously dispersed multimetal oxygen-evolving catalysts
Zhang, B., Zheng, X., Voznyy, O., Comin, R., Bajdich, M., García-Melchor, M., Han, L., Xu, J., Liu, M., Zheng, L., et al. (2016) · Science · doi:10.1126/science.aaf1525 · Cited by 2,447
Weng, B., Song, Z., Zhu, R., Yan, Q., Sun, Q., Grice, C. G., Yan, Y., & Yin, W.-J. (2020) · Nature Communications · doi:10.1038/s41467-020-17263-9 · Cited by 376
Cited by
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
Sun, H., Xu, X., Kim, H., Jung, W., Zhou, W., & Shao, Z. (2023) · ENERGY & ENVIRONMENTAL MATERIALS · doi:10.1002/eem2.12441 · Cited by 601
Self-citationZhong, H., Zhang, Q., Yu, J., Zhang, X., Wu, C., Ma, Y., An, H., Wang, H., Zhang, J., Wang, X., et al. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202301391 · Cited by 386
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Metadata
- Authors
- Xu, X., Pan, Y., Ge, L., Chen, Y., Mao, X., Guan, D., Li, M., Zhong, Y., Hu, Z., Peterson, V. K., Saunders, M., Chen, C., Zhang, H., Ran, R., Du, A., Wang, H., Jiang, S. P., Zhou, W., & Shao, Z.
- Venue
- Small
- Publisher
- Wiley
- Published
- 2021-06-17
- Volume
- 17
- Issue
- 29
- Pages
- e2101573-e2101573
- ISSN
- 1613-6810 (ISSN-L)
- 1613-6829
- OpenAlex
- W3170707030
- Cited by
- 238
- References
- 5
- FWCI
- 9.19
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xu, X., Pan, Y., Ge, L., Chen, Y., Mao, X., Guan, D., Li, M., Zhong, Y., Hu, Z., Peterson, V. K., Saunders, M., Chen, C., Zhang, H., Ran, R., Du, A., Wang, H., Jiang, S. P., Zhou, W., & Shao, Z. (2021). High‐Performance Perovskite Composite Electrocatalysts Enabled by Controllable Interface Engineering. Small. https://doi.org/10.1002/smll.202101573
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