Stable isotopes of carbon and oxygen for the study of carbonation/decarbonation processes in concretes
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During natural carbonation in ambient air and open systems, the heavier 13C isotopes are depleted in the solid phase.
“While accelerated aqueous carbonation at high CO2 concentrations in closed systems leads to an enrichment of the heavier ¹³C isotope in the solid phase, during natural carbonation in ambient air and open systems, the heavier ¹³C isotopes are depleted in the solid phase [33, 34, 41].”
From Isotope chemistry to trace carbon mineralization in construction materials (2026) · cites this paper as [41]
Accelerated aqueous carbonation at high CO2 concentrations in closed systems leads to an enrichment of the heavier 13C isotope in the solid phase.
“While accelerated aqueous carbonation at high CO2 concentrations in closed systems leads to an enrichment of the heavier ¹³C isotope in the solid phase, during natural carbonation in ambient air and open systems, the heavier ¹³C isotopes are depleted in the solid phase [33, 34, 41].”
From Isotope chemistry to trace carbon mineralization in construction materials (2026) · cites this paper as [41]
It is not always the case that δ13C values of carbonates formed during carbonation increase; some studies report that the δ13C value of the carbonated material decreases if carbonation occurs in ambient air.
“It is also not always the case that 𝛿 ¹³C values of carbonates formed during carbonation increase as shown in our experiments [38]. Instead, some studies report that the 𝛿 ¹³C value of the carbonated material decreases if the carbonation occurs in ambient air [33, 34, 41].”
From Isotope chemistry to trace carbon mineralization in construction materials (2026) · cites this paper as [41]
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- Authors
- Létolle, R., Gégout, P., Rafai, N., & Revertegat, E.
- Affiliations
- Université Pierre-et-Marie-Curie (FR)
- Venue
- Cement and Concrete Research
- Publisher
- Elsevier BV
- Published
- 1992-03
- Volume
- 22
- Issue
- 2-3
- Pages
- 235-240
- ISSN
- 0008-8846 (ISSN-L)
- OpenAlex
- W2093276173
- Cited by
- 24
- References
- 9
- Citations by year
- 2026: 3 · 2023: 2 · 2022: 1 · 2019: 1 · 2018: 2 · 2017: 4 · 2015: 2 · 2012: 1
- FWCI
- 2.38
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Cement and Concrete Research (publishedVersion)
- Topics
- Physical Sciences › Engineering › Civil and Structural Engineering › Concrete and Cement Materials Research
- Physical Sciences › Engineering › Civil and Structural Engineering › Concrete Corrosion and Durability
- Physical Sciences › Earth and Planetary Sciences › Earth-Surface Processes › Building materials and conservation
- Keywords
- stable carbon isotopes, stable oxygen isotopes, concrete carbonation, secondary carbonates, lime filler, CO2-saturated water
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