The mechanism of carbonate growth on concrete structures, as elucidated by carbon and oxygen isotope analyses
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Kinetic fractionation through aqueous carbonate speciation can become dominant and result in a δ13C depletion of -10 to -19‰ for hyper alkaline solutions.
“Specifically, kinetic fractionation through aqueous carbonate speciation (deprotonation of CO2(aq) to HCO3 -or CO 3 2) can become dominant and result in a 𝛿 ¹³C depletion of -10 to -19 ‰ for hyper alkaline solutions [46 -49].”
From Isotope chemistry to trace carbon mineralization in construction materials (2026) · cites this paper as [47]
Cites
The geochemistry of the stable carbon isotopes
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Thode, H. G., Shima, M., Rees, C. E., & Krishnamurty, K. V. (1965) · Canadian Journal of Chemistry · doi:10.1139/v65-076 · Cited by 121 · see citing works
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Hartmann, J., West, A. J., Renforth, P., Köhler, P., De La Rocha, C. L., Wolf‐Gladrow, D. A., Dürr, H. H., & Scheffran, J. (2013) · Reviews of Geophysics · doi:10.1002/rog.20004 · Cited by 717 · see citing works
Carbonate precipitation in artificial soils as a sink for atmospheric carbon dioxide
Renforth, P., Manning, D. A. C., & Lopez-Capel, E. (2009) · Applied Geochemistry · doi:10.1016/j.apgeochem.2009.05.005 · Cited by 161 · see citing works
Washbourne, C.-L., Renforth, P., & Manning, D. A. C. (2012) · Science of The Total Environment · doi:10.1016/j.scitotenv.2012.05.037 · Cited by 129 · see citing works
Rapid Removal of Atmospheric CO2 by Urban Soils
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Atmospheric CO2 Sequestration in Iron and Steel Slag: Consett, County Durham, United Kingdom
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Oxygen isotope fractionation in the CaCO3-DIC-H2O system
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Isotopic investigations of carbonate growth on concrete structures
Krishnamurthy, R. V., Schmitt, D., Atekwana, E. A., & Baskaran, M. (2003) · Applied Geochemistry · doi:10.1016/s0883-2927(02)00089-6 · Cited by 27 · see citing works
Létolle, R., Gégout, P., Rafai, N., & Revertegat, E. (1992) · Cement and Concrete Research · doi:10.1016/0008-8846(92)90061-y · Cited by 24 · see citing works
Isotope chemistry to trace carbon mineralization in construction materials
Jansen, D., Matschei, T., Van Geldern, R., Barth, J., & Snellings, R. (2026) · RILEM Technical Letters · doi:10.21809/rilemtechlett.2026.232
- Authors
- Macleod, G., Fallick, A. E., & Hall, A. J.
- Affiliations
- University of Glasgow (GB)
- ORCID
- Fallick, A.E.
- Venue
- Chemical Geology: Isotope Geoscience section
- Publisher
- Elsevier BV
- Published
- 1991-04
- Volume
- 86
- Issue
- 4
- Pages
- 335-343
- ISSN
- 0168-9622 (ISSN-L)
- OpenAlex
- W1975415136
- Cited by
- 35
- References
- 3
- Citations by year
- 2026: 1 · 2023: 1 · 2022: 1 · 2020: 2 · 2019: 1 · 2018: 3 · 2017: 3 · 2015: 3 · 2014: 1 · 2013: 1 · 2012: 2
- FWCI
- 0.38
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Chemical Geology Isotope Geoscience section (publishedVersion)
- Funders
- Natural Environment Research Council
- Topics
- Physical Sciences › Materials Science › Biomaterials › Calcium Carbonate Crystallization and Inhibition
- Physical Sciences › Earth and Planetary Sciences › Earth-Surface Processes › Building materials and conservation
- Physical Sciences › Engineering › Civil and Structural Engineering › Concrete and Cement Materials Research
- Keywords
- calcite, stalactites, carbon isotope fractionation, oxygen isotope fractionation, atmospheric CO2, portlandite dissolution, gas-liquid interface, concrete structures, Midland Valley of Scotland
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