Effect of pressure on the electrochemical reduction of CO2 on Group VIII metal electrodes
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While the dominant products of CO2RR do not change significantly with temperature on most catalysts, studies on Cu have demonstrated that hydrocarbon selectivity tends to shift from CH4 to C2H4 as temperature increases.
“While the dominant products of CO2RR do not change significantly with temperature on most catalysts, [240] studies on Cu have demonstrated that hydrocarbon selectivity tends to shift from CH4 to C2H4 as temperature increases.[242,[245][246][247]”
From Electrochemical CO <sub>2</sub> Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design (2019) · cites this paper as [240]
Improved C2H4 selectivity with increasing temperature is attributed to reduced activation energies and enhanced surface diffusion of adsorbed intermediates.
“This improved C2H4 selectivity is attributed to reduced activation energies [240] and enhanced surface diffusion of adsorbed intermediates.[242]”
From Electrochemical CO <sub>2</sub> Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design (2019) · cites this paper as [240]
In H cell reactors, the increased CO2 solubility achieved at lower temperatures improves the selectivity for CO2RR as compared to the HER.
“In these systems, the increased CO2 solubility achieved at lower temperatures (Figure .13) improves the selectivity for CO2RR as compared to the HER.[239][240][241][242][243][244]”
From Electrochemical CO <sub>2</sub> Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design (2019) · cites this paper as [240]
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A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
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Electrocatalysis for CO <sub>2</sub> conversion: from fundamentals to value-added products
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Operation of a Pressurized System for Continuous Reduction of CO<sub>2</sub>
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Large Current Density CO2 Reduction under High Pressure Using Gas Diffusion Electrodes
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- Authors
- Nakagawa, S., Kudo, A., Azuma, M., & Sakata, T.
- Affiliations
- Tokyo Institute of Technology (JP)
- Corresponding author
- Sakata, Tadayoshi
- ORCID
- Kudo, Akihiko
- Venue
- Journal of Electroanalytical Chemistry and Interfacial Electrochemistry
- Publisher
- Elsevier BV
- Published
- 1991-06
- Volume
- 308
- Issue
- 1-2
- Pages
- 339-343
- ISSN
- 0022-0728 (ISSN-L)
- OpenAlex
- W1970877213
- Cited by
- 86
- References
- 14
- Citations by year
- 2026: 2 · 2025: 4 · 2024: 2 · 2023: 3 · 2022: 2 · 2021: 7 · 2020: 3 · 2019: 6 · 2018: 3 · 2017: 6 · 2016: 5 · 2015: 4 · 2014: 6 · 2013: 3 · 2012: 1
- FWCI
- 2.11
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Electroanalytical Chemistry (publishedVersion)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Keywords
- electrochemical CO2 reduction, high pressure, iron, cobalt, nickel, palladium, platinum
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