Comparative kinetics study on carbonation of ettringite and meta-ettringite based materials
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In carbonated Y-A paste, only bassanite is observed as the calcium sulphate crystalline phase because the RH of the carbonation experiment was 65%.
“In agreement with previous reports [18,19,21], only bassanite is observed here, as calcium sulphate crystalline phase, because the RH of the carbonation experiment was 65%.”
From X-ray Total Scattering Study of Phases Formed from Cement Phases Carbonation (2021) · cites this paper as [18]
Section 4.6.2 (page unavailable) reports hemihydrate rather than gypsum in an ettringite-based material carbonated at 65% RH, and explains how moisture conditions can favor hemihydrate. It does not report observations in Y-A paste; its own hydrated samples at 70% RH contained both hemihydrate and trace gypsum. Thus it supports the comparison, but not the claim that 65% RH explains the exclusive observation in Y-A paste. (LLM, conf=0.86)
Experimental — accuracy not yet measuredGypsum is formed at high RH values of ~90% while bassanite forms at lower RH (e.g., 60-70%).
“It is well established that gypsum is formed at high RH values of ~90% meanwhile bassanite forms at lower RH (e.g., 60-70%) [18,19,21].”
From X-ray Total Scattering Study of Phases Formed from Cement Phases Carbonation (2021) · cites this paper as [18]
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Saeki, N., Kurihara, R., Ohkubo, T., Teramoto, A., Suda, Y., Kitagaki, R., & Maruyama, I. (2025) · Cement and Concrete Research · doi:10.1016/j.cemconres.2024.107777 · Cited by 48 · see citing works
X-ray Total Scattering Study of Phases Formed from Cement Phases Carbonation
Cuesta, A., De la Torre, A. G., & Aranda, M. A. G. (2021) · Minerals · doi:10.3390/min11050519 · Cited by 14 · see citing works
“Calcium carbonate polymorph formation seems to depend upon the carbonation conditions with works reporting aragonite [16,19], vaterite [20], mixtures of vaterite and aragonite [18], calcite [17] and even the three CaCO3 polymorphs depending upon the investigated sample [15].”
BackgroundMethod
- Authors
- Chen, B., Horgnies, M., Huet, B., Morin, V., Johannes, K., & Kuznik, F.
- Affiliations
- Lyon 1 Université (FR)
- LafargeHolcim (France) (FR)
- Corresponding author
- Chen, Bao
- Venue
- Cement and Concrete Research
- Publisher
- Elsevier BV
- Published
- 2020-11
- Volume
- 137
- Pages
- 106209
- ISSN
- 0008-8846 (ISSN-L)
- OpenAlex
- W3084217029
- Cited by
- 76
- References
- 41
- Citations by year
- 2026: 12 · 2025: 21 · 2024: 24 · 2023: 7 · 2022: 6 · 2021: 4 · 2020: 2
- FWCI
- 2.34
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Cement and Concrete Research (acceptedVersion)
- HAL (submittedVersion, cc-by-nc)
- Funders
- Association Nationale de la Recherche et de la Technologie
- Topics
- Physical Sciences › Engineering › Mechanical Engineering › Adsorption and Cooling Systems
- Physical Sciences › Engineering › Civil and Structural Engineering › Concrete and Cement Materials Research
- Physical Sciences › Materials Science › Materials Chemistry › Thermal and Kinetic Analysis
- Keywords
- ettringite, carbonation kinetics, calcium aluminate cement, ordinary Portland cement, relative humidity, CO2 concentration, vaterite, aragonite, calcium sulfate hemihydrate, gypsum, heat storage capacity
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