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Carbonate precipitation in artificial soils produced from basaltic quarry fines and composts: An opportunity for passive carbon sequestration
Open accessAbstract
The proportions of different carbon pools within artificial soils prepared by blending composts with dolerite and basalt quarry fines has changed over a period of 7 years, accumulating inorganic carbon as carbonate minerals newly formed within the soils. With no artificial energy inputs following construction, this is regarded as a passive mineral carbonation process. Carbon isotope data show that up to 40% of the carbon within the soil carbonate is derived from photosynthesis, mixed with carbon from geological sources (limestone present in the quarry fines). Organic matter within the soils shows very variable composition, with an apparent increase with time in the relative proportion of labile carbon relative to more stable forms, reflecting a change in the soil organic matter composition associated with the establishment of new plant communities. The rate of accumulation of inorganic carbon as carbonate minerals is estimated to be equivalent to 4.8 t C ha−1 annually to a depth of 0.3 m, consistent with rates observed for accumulations of carbonate carbon in urban soils containing demolition wastes (annually 3.0 t C ha−1 to 0.3 m). There appears to be substantial potential for artificial soils to be designed expressly for the purpose of carbon capture. The process is analogous to the use of reed beds for the removal of pollutants from contaminated waters.
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“Similar observations have been found at other sites, where the rate of CO 2 removal has been estimated on the basis of the assumption that calcium carbonate content in soil was zero at the time of demolition 9 or soil formation.14”
From Rapid Removal of Atmospheric CO2 by Urban Soils (2015) · cites this paper as [14]
In the citing paper
“Although reported here for urban soils with artificial mineral inputs, calcite precipitation has also been observed in artificial soils prepared by blending natural calcium silicate rocks with compost.14”
From Rapid Removal of Atmospheric CO2 by Urban Soils (2015) · cites this paper as [14]
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“Carbonation appears to decrease with depth, likely due to the isolation of materials from the atmosphere; therefore, management that increases atmospheric exposure (e.g., through appropriate planting that takes CO 2 to depth via plant root systems and associated metabolism) is likely to increase carbonation rates throughout the site.14,45,46”
From Rapid Removal of Atmospheric CO2 by Urban Soils (2015) · cites this paper as [14]
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Korchagin, J. (2018) · theses.fr (ABES) · doi:10.70675/23fe0fddz70a0z476az9480z5dbf63781441 · Cited by 1
Rohling, E. J. (2021) · doi:10.1093/oso/9780197502556.003.0004
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Rodrigues, B. M. (2023) · Digital Library of Theses and Dissertations (Universidade de São Paulo) · doi:10.11606/t.11.2023.tde-05062023-144454
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Metadata
- Authors
- Manning, D. A. C., Renforth, P., Lopez-Capel, E., Robertson, S., & Ghazireh, N.
- Affiliations
- Newcastle University (GB)
- University of Oxford (GB)
- Durham University (GB)
- Corresponding author
- Manning, D.A.C.
- Venue
- International journal of greenhouse gas control
- Publisher
- Elsevier BV
- Published
- 2013-09
- Volume
- 17
- Pages
- 309-317
- ISSN
- 1750-5836 (ISSN-L)
- OpenAlex
- W2131652913
- Cited by
- 106
- References
- 56
- Citations by year
- 2026: 6 · 2025: 10 · 2024: 16 · 2023: 15 · 2022: 10 · 2021: 9 · 2020: 10 · 2019: 11 · 2018: 4 · 2017: 6 · 2016: 4 · 2015: 4 · 2014: 1
- FWCI
- 4.34
- Type
- journal article
- Language
- en
- Open access
- hybrid
- doi.org
- Licence
- Locations
- International journal of greenhouse gas control (publishedVersion, cc-by)
- ORCA Online Research @Cardiff (Cardiff University) (submittedVersion)
- Newcastle University ePrints (Newcastle Univesity) (cc-by)
- Funders
- Engineering and Physical Sciences Research Council (EP/F02777X/1)
- Topics
- Life Sciences › Agricultural and Biological Sciences › Soil Science › Soil Carbon and Nitrogen Dynamics
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Life Sciences › Agricultural and Biological Sciences › Soil Science › Soil and Environmental Studies
- Keywords
- carbonate precipitation, CO2 mineralization, artificial soil, compost, soil organic matter, labile carbon, carbon isotope analysis, diabase, demolition waste, urban soils, CO2 capture
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